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Article
Asymmetrical π back-donation of hetero-dicationic Mo4+-Mo6+ pairs for enhanced electrochemical nitrogen reduction
The breaking of nonpolar N≡N bond of dinitrogen is the biggest dilemma for electrocatalytic nitrogen reduction reaction (NRR) application, driving electron migration between catalysts and N≡N bond (termed “π b...
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Article
Open AccessEngineering a local acid-like environment in alkaline medium for efficient hydrogen evolution reaction
Tuning the local reaction environment is an important and challenging issue for determining electrochemical performances. Herein, we propose a strategy of intentionally engineering the local reaction environme...
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Article
Open AccessIntrinsic room-temperature ferromagnetism in a two-dimensional semiconducting metal-organic framework
The development of two-dimensional (2D) magnetic semiconductors with room-temperature ferromagnetism is a significant challenge in materials science and is important for the development of next-generation spin...
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Article
Open AccessDual-site segmentally synergistic catalysis mechanism: boosting CoFeSx nanocluster for sustainable water oxidation
Efficient oxygen evolution reaction electrocatalysts are essential for sustainable clean energy conversion. However, catalytic materials followed the conventional adsorbate evolution mechanism (AEM) with the i...
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Article
Classical spin liquid state in a rhombic lattice metal-organic framework
Discovering more and new geometrically frustrated systems remains an active point of inquiry in fundamental physics for the existence of unusual states of matter. Here, we report spin-liquid-like behavior in a...
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Article
Dual-terminal artificial synapse in two-dimensional CrSBr memristor for neuromorphic computing
Novel computing technologies that imitate the principles of biological neural systems may serve low power consumption with significant cognitive and learning advantages. The development of memristors with non-...