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Article
Open AccessActinium chelation and crystallization in a macromolecular scaffold
Targeted alpha therapy (TAT) pairs the specificity of antigen targeting with the lethality of alpha particles to eradicate cancerous cells. Actinium-225 [225Ac; t1/2 = 9.920(3) days] is an alpha-emitting radioiso...
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Article
Open AccessImpeding 99Tc(IV) mobility in novel waste forms
Technetium (99Tc) is an abundant, long-lived radioactive fission product whose mobility in the subsurface is largely governed by its oxidation state. Tc immobilization is crucial for radioactive waste management ...
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Article
Tc and Re Behavior in Borosilicate Waste Glass Vapor Hydration Tests
Technetium (Tc), found in some nuclear wastes, is of particular concern with regard to long-term storage, because of its long-lived radioactivity and high mobility in the environment. Tc and rhenium (Re), comm...
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Article
X-ray Absorption Fine Structure Studies of Speciation of Technetium in Borosilicate Glasses
A series of glass samples were prepared analogously to high level waste glass using either glass frit or glass precursors combined with a high level waste surrogate containing NaTcO4. Three different technetium s...