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Article
Chemical interface dam** of surface plasmon excitation in metal nanoparticles: a study by persistent spectral hole burning
As demonstrated recently, persistent spectral hole burning in the optical spectra of metal nanoparticles makes possible the determination of the ultrafast dephasing time T2 of surface plasmon excitation. Here, th...
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Article
Application of metal nanoparticles in confocal laser scanning microscopy: improved resolution by optical field enhancement
We describe experiments in which the field enhancement by metal nanoparticles that accompanies surface plasmon excitation has been exploited in confocal laser scanning microscopy. The objective was to make use...
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Article
Spectral hole burning in absorption profiles of metal nanoparticles prepared by laser assisted growth
We have combined two novel methods, i.e. persistent spectral hole burning and laser assisted growth, to measure the decay time T2 of surface plasmon excitation in metal nanoparticles of different size at constant...
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Article
Theory of spectral hole burning for the study of ultrafast electron dynamics in metal nanoparticles
In order to study the ultrafast relaxation dynamics of surface plasmon excitation in metal nanoparticles in the presence of inhomogeneous line broadening and investigate the influence of the reduced dimensions...
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Article
Laser manipulation of the size and shape of supported nanoparticles
Laser manipulation of the size and shape of metal nanoparticles prepared by self assembly of atoms on dielectric surfaces is discussed. The technique relies on the optical properties of the aggregates and the ...
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Article
Silicon nanoclusters formed through self-assembly on CaF2 substrates: morphology and optical properties
We studied the influence of the size and shape of silicon nanoclusters on their optical response. For this purpose, clusters were prepared by deposition, and subsequent diffusion and nucleation, of Si atoms on...
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Article
Laser-induced manipulation of the size and shape of small metal particles: Towards monodisperse clusters on surfaces
A novel experimental technique is presented for post growth narrowing of the size distribution of metal nanoparticles on dielectric substrates. In order to demonstrate the potential of the method, oblate Ag cl...
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Article
Sha** nanoparticles and their optical spectra with photons
An experimental method to tailor the shape and the optical absorption spectra of metallic nanoparticles is presented. It exploits the influence of laser irradiation on particle growth by self-assembly of atoms...
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Article
Formation of gold nanowires through self-assembly during scanning force microscopy
Gold films with a nominal thickness of 5–40 monolayers were grown on dielectric substrates and imaged by scanning force microscopy (SFM). The films originally consisted of well-separated or densely packed clus...
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Chapter and Conference Paper
Laser-induced manipulation of the size and shape of small metal particles: Towards monodisperse clusters on surfaces
A novel experimental technique is presented for post growth narrowing of the size distribution of metal nanoparticles on dielectric substrates. In order to demonstrate the potential of the method, oblate Ag cl...
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Article
Adsorbate-induced transition between different mechanisms of laser-stimulated desorption
were measured as a function of laser fluence, number of laser pulses, and oxygen exposure. If the laser fluence exceeds 10 mJ/cm2 desorption from clean particles occurs as a thermal reaction. Oxygen exposure as ...
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Article
Influence of molecular adsorbate layers on the optical spectra of small metal particles
, N2O, CO2 or N2 on the particle surface. Depending on the molecules to which the clusters are exposed, different changes of the surface plasmon resonance in the spectra can be identified. The most essential expe...