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Water contents in aggregates and cement pastes determined by gravimetric analysis and prompt γ-ray analysis

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Abstract

We determined the free + adsorbed water and the bound water in aggregates and cement pastes using conventional gravimetric analysis and prompt γ-ray analysis, respectively, to evaluate the total water content in concretes. The contents of free + adsorbed water and bound water in some geochemical references were also determined to confirm the accuracy in the present work. The content of each water in aggregates collected from different quarries and cement pastes with different water-to-cement ratios were analyzed. The total water content in young concrete was evaluated on the basis of the analytical values.

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References

  1. Goorley T, James M, Booth T, Brown F, Bull J, Cox LJ, Durkee J, Elson J, Fensin M, Forster RA, Hendricks J, Hughes HG, Johns R, Kiedrowski B, Martz R, Mashnik S, McKinney G, Pelowitz D, Prael R, Sweezy J, Waters L, Wilcox T, Zukaitis T (2012) Initial MCNP6 release overview. Nucl Technol 180:298–315

    Article  CAS  Google Scholar 

  2. Oak Ridge National Laboratory SCALE Version 44 A Modular Code System for performing standardized computer analyses for licensing evaluation, NUREG/CR-0200 Rev 6 ORNL/NUREG/CSD-2/1R6 vol 2 Part 1, Published May 2000. https://www.nrc.gov/docs/ML0037/ML003722257.pdf. Accessed 21 Sep 2022

  3. Kosako K, Oishi K, Nakamura T, Sato K, Kamiyama K, Kiyanagi Y (2013) Shielding study on iron and concrete assemblies of bremsstrahlung photons and photoneutrons from copper target bombarded by 18, 28 and 38 MeV electrons. J Nucl Sci Technol 50:1188–1197

    Article  CAS  Google Scholar 

  4. Kinoshita N, Noto T, Kosako K, Torii K, Tada A, Urabe K, Outsuki T, Sekimoto S (2021) Uncertainty derived from elemental analysis and its effect on the separation of radioactive waste into low-level radioactive waste and waste for clearance. Prog Nucl Energy 131:103597

    Article  CAS  Google Scholar 

  5. Kinoshita N, Noto T, Kosako K, Asada M, Urabe K, Tada A, Tori K (2019) Boundary depth between LLRW and CLW affected by fluctuation of elemental composition. In: Proceedings of the 25th conference on structural mechanics in reactor technology (SMiRT-25) Charlotte NC. 4–9 Aug 2019

  6. Zhang R, **ao Y, Wu M, Zheng J, Milkos BC (2021) Measurement and engineering application of adsorbed water content in fine-grained soils. J Cent South Univ 28:1555–1569

    Article  Google Scholar 

  7. Yuan Y, Rezaee R, Verrall M, Hu S, Zou J, Testmanti N (2018) Pore characterization and clay bound water assessment in shale with a combination of NMR and low-pressure nitrogen gas adsorption. Int J Coal Geol 194:11–21

    Article  CAS  Google Scholar 

  8. Santha KG (2019) Influence of fluidity on mechanical and permeation performances of recycled aggregate mortar. Constr Build Mater 213:404–412

    Article  Google Scholar 

  9. Lura P, Winnefeld F, Fang XJ (2017) A simple method for determining the total amount of physically and chemically bound water of different cements. Therm Anal Calorim 130:653–660

    Article  CAS  Google Scholar 

  10. Khorami J, Lemieux A (1989) Comparison of attapulgites from different sources using TG/DTG and FTIR. Themochim Acta 138:97–105

    Article  CAS  Google Scholar 

  11. Lee DJ, Hsu YH (1995) Measurement of bound water in sludges: a comparative study. Water Environ Res 67:310–317

    Article  CAS  Google Scholar 

  12. Wang Y, Lu S, Ren T, Li B (2011) Bound water content of air-dry soils measured by thermal analysis. Soil Sci Soc Am J 75:481–487

    Article  CAS  Google Scholar 

  13. Terashima S (1979) The determination of major and minor elements on the two geochemical reference samples, JA-1 and JB-2 and six geochemical exploration reference samples. Bull Geol Surv Jpn 30:37–43

    CAS  Google Scholar 

  14. Lindstrom RM, Révay ZJ (2017) Prompt gamma neutron activation analysis (PGAA): recent developments and applications. Radioanal Nucl Chem 314:843–858

    Article  CAS  Google Scholar 

  15. Kino K, Furusaka M, Hiraga F, Kamiyama T, Kiyanagi Y, Furutaka K, Goko S, Harada H, Harada M, Kai T, Kimura A, Kin T, Kitatani F, Koizumi M, Maekawa F, Meigo S, Nakamura S, Ooi M, Ohta M, Oshima M, Toh Y, Igashira M, Katabuchi T, Mizumoto M (2011) Measurement of energy spectra and spatial distributions of neutron beams provided by the ANNRI beamline for capture cross-section measurements at the J-PARC/MLF. Nucl Instrum Meth B 626–627:58–66

    Article  Google Scholar 

  16. Toh Y, Ebihara M, Kimura A, Nakamura S, Harada H, Hara KY, Koizumi M, Kitatani F, Furutaka K (2014) Synergistic effect of combining two nondestructive analytical methods for multielemental analysis. Anal Chem 86:12030–12036

    Article  CAS  Google Scholar 

  17. Shen W, Li X, Lu X, Guo W, Zhou S, Wan Y (2018) Experimental study and isotherm models of water vapor adsorption in shale rocks. J Nat Gas Sci Eng 52:484–491

    Article  CAS  Google Scholar 

  18. Toh Y, Segawa M, Maeda M, Tsuneyama M, Kimura A, Nakamura S, Endo S, Ebihara M (2021) Nondestructive quantitative analysis of difficult-to-measure radionuclides 107Pd and 99Tc. Anal Chem 93:9771–9777

    Article  CAS  Google Scholar 

  19. Kimura A, Toh Y, Koizumi M, Osa A, Oshima M, Goto J, Igashira M (2005) Development of a data acquisition system for a multiple gamma-ray detection method. AIP Conf Proc 769:792–795

    Article  Google Scholar 

  20. Kimura A, Toh Y, Koizumi M, Furutaka K, Kin T, Oshima M (2008) Performance of a high speed and high density data acquisition system for multiple γ-ray detection. IEEE Nucl Sci Symp Conf Rec 2107–2111

  21. Iwamoto O, Iwamoto N, Shibata K, Ichihara A, Kunieda S, Minato F, Nakayama S (2020) Status of JENDL. EPJ Web Conf 239:09002

    Article  CAS  Google Scholar 

  22. Imai N, Terashima S, Itoh S, Ando A (1995) 1994 compilation of analytical data for minor and trace elements in seventeen GSJ geochemical reference samples, “igneous rock series.” Geostand Newsl 19:135–213

    Article  CAS  Google Scholar 

  23. Hasterok D, Webb J (2017) On the radiogenic heat production of igneous rocks. Geosci Front 8:919–940

    Article  CAS  Google Scholar 

  24. Liu Z, Xu D, Zhang Y (2017) Experimental investigation and quantitative calculation of the degree of hydration and products in fly ash-cement mixtures. Adv Mater Sci Eng 2437270

  25. Liao W, Sun X, Kumar A, Sun H, Ma H (2019) Hydration of binary Portland cement blends containing silica fume: a decoupling method to estimate degrees of hydration and pozzolanic reaction. Front Mater 6:78

    Article  Google Scholar 

  26. Baroghel-Bouny V, Mainguy M, Lassabatere T, Coussy O (1999) Characterization and identification of equilibrium and transfer moisture properties for ordinary and high-performance cementitious materials. Cem Concr Res 29:1225–1238

    Article  CAS  Google Scholar 

  27. Espinosa RM, Franke L (2006) Influence of the age and drying process on pore structure and sorption isotherms of hardened cement paste. Cem Concr Res 36:1969–1984

    Article  CAS  Google Scholar 

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Acknowledgements

The authors would like to thank staff of J-PARC/MLF for operation of the accelerator and supporting the PGA measurement. The PGA measurement was performed under the user program (Proposal No. 2021B0107).

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Correspondence to Norikazu Kinoshita.

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Kinoshita, N., Noto, T., Nakashima, H. et al. Water contents in aggregates and cement pastes determined by gravimetric analysis and prompt γ-ray analysis. J Radioanal Nucl Chem 332, 479–486 (2023). https://doi.org/10.1007/s10967-023-08776-w

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