Abstract
Stretchable conductors are indispensable components of stretchable electronic devices, such as stretchable sensors, transistors, light-emitting diode arrays, solar cells, and so on. However, most of the conductive materials are stiff with very low stretchability. Nature has evolved various strategies to realize stretchability, which give a lot of inspirations to the design and fabrication of stretchable conductors. We herein summarized the nature’s strategies to realize stretchability and revealed the underlying mechanisms. After that, the applications of these strategies in fabricating stretchable conductors are exemplified and the effects of some important parameters on the performances are discussed. Then, possible applications of these stretchable conductors are summarized. Finally, critical issues in the stretchable conductors are discussed and several prospective exploration directions are provided.
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Wang C. Y., Yokota T., Someya T., Chem. Rev., 2021, 121(4), 2109
Qi D., Zhang K., Tian G., Jiang B., Huang Y., Adv. Mater., 2021, 33(6), 2003155
Kim D. W., Kong M., Jeong U., Adv. Sci., 2021, 8(8), 2004170
Xue Z., Song H., Rogers J. A., Zhang Y., Huang Y., Adv. Mater., 2020, 32(15), 1902254
Wang T., Wang M., Yang L., Li Z., Loh X. J., Chen X., Adv. Mater., 2020, 32(8), 1905522
Wang P., Hu M., Wang H., Chen Z., Feng Y., Wang J., Ling W., Huang Y., Adv. Sci., 2020, 7(20), 2001116
Sim K., Rao Z. Y., Ershad F., Yu C. J., Adv. Mater., 2020, 32(15), 1902417
Yang J. C., Mun J., Kwon S. Y., Park S., Bao Z., Park S., Adv. Mater., 2019, 31(48), 1904765
Karipoth P., Christou A., Pullanchiyodan A., Dahiya R., Adv. Intell. Syst., 2021, 4(2), 2100092
Chen B., Shao Z., **e Z., Liu J., Pan F., He L., Zhang L., Zhang Y., Ling X., Peng F., Yun W., Wen L., Adv. Intell. Syst., 2021, 3(10), 2000251
McLellan K., Yoon Y., Leung S. N., Ko S. H., Adv. Mater. Technol., 2020, 5(4), 1900939
Lee J., Zambrano B. L., Woo J., Yoon K., Lee T., Adv. Mater., 2020, 32(5), 1902532
Zhao Y., Kim A., Wan G. X., Tee B. C. K., Nano Converg., 2019, 6(1), 25
Matsuhisa N., Chen X. D., Bao Z. A., Someya T., Chem. Soc. Rev., 2019, 48(11), 2946
Lee H. R., Kim C. C., Sun J. Y., Adv. Mater., 2018, 30(42), 1704403
Yang C., Suo Z., Nat. Rev. Mater., 2018, 3(6), 125
Yuk H., Lu B., Zhao X., Chem. Soc. Rev., 2019, 48(6), 1642
Huneau B., Rubber Chem. Technol., 2011, 84(3), 425
Neuefeind J., Skov A. L., Daniels J. E., Honkimäki V., Jakobsen B., Oddershede J., Poulsen H. F., RSC Adv., 2016, 6(98), 95910
Wang Y., Zhu C. X., Pfattner R., Yan H. P., ** L. H., Chen S. C., Molina-Lopez F., Lissel F., Liu J., Rabiah N. I., Chen Z., Chung J. W., Linder C., Toney M. F., Murmann B., Bao Z., Sci. Adv., 2017, 3(3), e1602076
Zheng Y. Q., Liu Y., Zhong D., Nikzad S., Liu S., Yu Z., Liu D., Wu H. C., Zhu C., Li J., Tran H., Tok J. B., Bao Z., Science, 2021, 373(6550), 88
Wessendorf A. M., Newman D. J., IEEE Trans. Biomed. Eng., 2012, 59(12), 3432
Gerbode S. J., Puzey J. R., McCormick A. G., Mahadevan L., Science, 2012, 337(6098), 1087
Cheng Y., Wang R., Chan K. H., Lu X., Sun J., Ho G. W., ACS Nano, 2018, 12(4), 3898
Godinho M. H., Canejo J. P., Feio G., Terentjev E. M., Soft Matter, 2010, 6(23), 5965
Wang J. S., Wang G., Feng X. Q., Kitamura T., Kang Y. L., Yu S. W., Qin Q. H., Sci. Rep., 2013, 3, 3102
Zhao Y., Miao X., Lin J., Li X., Bian F., Wang J., Zhang X., Yue B., Glob. Chall., 2017, 1(3), 1600021
Yang Z., Zhai Z., Song Z., Wu Y., Liang J., Shan Y., Zheng J., Liang H., Jiang H., Adv. Mater., 2020, 32, 1907495
Harrington M. J., Razghandi K., Ditsch F., Guiducci L., Rueggeberg M., Dunlop J. W. C., Fratzl P., Neinhuis C., Burgert I., Nat. Commun., 2011, 2, 337
Zhang F., Jiang L., Wang S., Proc. Natl. Acad. Sci., 2018, 115(40), 10046
Wang C., Lv Z., Mohan M. P., Cui Z., Liu Z., Jiang Y., Li J., Wang C., Pan S., Karim M. F., Liu A. Q., Chen X., Adv. Mater., 2021, 33(41), 2102131
Wang B., Yang W., Sherman V. R., Meyers M. A., Acta Biomater., 2016, 41, 60
Lv Z., Wang C., Wan C., Wang R., Dai X., Wei J., **a H., Li W., Zhang W., Cao S., Zhang F., Yang H., Loh X. J., Chen X., Adv. Mater., 2022, 34, 2202877
Qi D. P., Liu Z. Y., Liu Y., Jiang Y., Leow W. R., Pal M., Pan S. W., Yang H., Wang Y., Zhang X. Q., Yu J. C., Li B., Yu Z., Wang W., Chen X. D., Adv. Mater., 2017, 29(40), 1702800
Lang U., Naujoks N., Dual J., Synth. Met., 2009, 159(5/6), 473
Teo M. Y., Kim N., Kee S., Kim B. S., Kim G., Hong S., Jung S., Lee K., ACS Appl. Mater. Interfaces, 2017, 9(1), 819
Lee J. H., Jeong Y. R., Lee G., ** S. W., Lee Y. H., Hong S. Y., Park H., Kim J. W., Lee S. S., Ha J. S., ACS Appl. Mater. Interfaces, 2018, 10(33), 28027
Vosgueritchian M., Lipomi D. J., Bao Z. A., Adv. Funct. Mater., 2012, 22(2), 421
Palumbiny C. M., Liu F., Russell T. P., Hexemer A., Wang C., Muller-Buschbaum P., Adv. Mater., 2015, 27(22), 3391
Liu D., Osuna Orozco R., Wang T., Phys. Rev. E, 2013, 88(2), 022601
Feig V. R., Tran H., Lee M., Bao Z., Nat. Commun., 2018, 9(1), 2740
Kayser L. V., Lipomi D. J., Adv. Mater., 2019, 31(10), 1806133
Liu Y., Li J., Song S., Kang J., Tsao Y., Chen S., Mottini V., McConnell K., Xu W., Zheng Y. Q., Tok J. B., George P. M., Bao Z., Nat. Biotechnol., 2020, 38(9), 1031
Alemu Mengistie D., Wang P.-C., Chu C.-W., J. Mater. Chem. A, 2013, 1(34), 9907
Shi H., Liu C., Jiang Q., Xu J., Adv. Electron. Mater., 2015, 1(4), 1500017
Oh J. Y., Rondeau-Gagne S., Chiu Y. C., Chortos A., Lissel F., Wang G. N., Schroeder B. C., Kurosawa T., Lopez J., Katsumata T., Xu J., Zhu C., Gu X., Bae W. G., Kim Y., ** L., Chung J. W., Tok J. B., Bao Z., Nature, 2016, 539(7629), 411
Xu J., Wang S., Wang G. N., Zhu C., Luo S., ** L., Gu X., Chen S., Feig V. R., To J. W., Rondeau-Gagne S., Park J., Schroeder B. C., Lu C., Oh J. Y., Wang Y., Kim Y. H., Yan H., Sinclair R., Zhou D., Xue G., Murmann B., Linder C., Cai W., Tok J. B., Chung J. W., Bao Z., Science, 2017, 355(6320), 59
Xu J., Wu H. C., Zhu C., Ehrlich A., Shaw L., Nikolka M., Wang S., Molina-Lopez F., Gu X., Luo S., Zhou D., Kim Y. H., Wang G. N., Gu K., Feig V. R., Chen S., Kim Y., Katsumata T., Zheng Y. Q., Yan H., Chung J. W., Lopez J., Murmann B., Bao Z., Nat. Mater., 2019, 18(6), 594
Müller C., Goffri S., Breiby D. W., Andreasen J. W., Chanzy H. D., Janssen R. A. J., Nielsen M. M., Radano C. P., Sirringhaus H., Smith P., Stingelin-Stutzmann N., Adv. Funct. Mater., 2007, 17(15), 2674
Wilhelmi B. J., Blackwell S. J., Mancoll J. S., Phillips L. G., Ann. Plast. Surg., 1998, 41(2), 215
Gorrn P., Cao W. Z., Wagner S., Soft Matter, 2011, 7(16), 7177
Lipomi D. J., Tee B. C. K., Vosgueritchian M., Bao Z. N., Adv. Mater., 2011, 23(15), 1771
Wang X. L., Hu H., Shen Y. D., Zhou X. C., Zheng Z. J., Adv. Mater., 2011, 23(27), 3090
Lee P., Lee J., Lee H., Yeo J., Hong S., Nam K. H., Lee D., Lee S. S., Ko S. H., Adv. Mater., 2012, 24(25), 3326
Polywka A., Jakob T., Stegers L., Riedl T., Gorrn P., Adv. Mater., 2015, 27(25), 3755
Zhao Y. M., Dong D. S., Gong S., Brassart L., Wang Y., An T., Cheng W. L., Adv. Electron. Mater., 2019, 5(1), 1800462
Lee S., Song Y., Ko Y., Ko Y., Ko J., Kwon C. H., Huh J., Kim S. W., Yeom B., Cho J., Adv. Mater., 2020, 32(7), 1906460
Yang Y. H., Duan S., Zhao H., Adv. Mater. Interfaces, 2021, 8(9), 2100137
Bowden N., Brittain S., Evans A. G., Hutchinson J. W., Whitesides G. M., Nature, 1998, 393(6681), 146
Efimenko K., Rackaitis M., Manias E., Vaziri A., Mahadevan L., Genzer J., Nat. Mater., 2005, 4(4), 293
Yang S., Khare K., Lin P.-C., Adv. Funct. Mater., 2010, 20(16), 2550
Brau F., Damman P., Diamant H., Witten T. A., Soft Matter, 2013, 9(34), 8177
Li F., Hou H., Yin J., Jiang X., Sci. Adv., 2018, 4(4), eaar5762
Lee P., Ham J., Lee J., Hong S., Han S., Suh Y. D., Lee S. E., Yeo J., Lee S. S., Lee D., Ko S. H., Adv. Funct. Mater., 2014, 24(36), 5671
Won J., Mondal S., Park J., Wang W., Lee H., Kim S., Shin B., Sathi S. G., Nah C., Polym. Compos., 2020, 41(6), 2210
Liu Z., Wang H., Huang P., Huang J., Zhang Y., Wang Y., Yu M., Chen S., Qi D., Wang T., Jiang Y., Chen G., Hu G., Li W., Yu J., Luo Y., Loh X. J., Liedberg B., Li G., Chen X., Adv. Mater., 2019, 31(35), 1901360
García-Gallegos J. H., Nieto-Navarro J. G., Araujo-Palomo E. E., Zamora-Antuñano M. A., Olivares-Ramírez J. M., Encinas A., Mater. Lett., 2014, 115, 100
Zhou J., Tian G. Q., ** G., **n Y. Y., Tao R., Lubineau G., Adv. Funct. Mater., 2020, 30(5), 1907316
Yu Y., Zhang Y. K., Li K., Yan C., Zheng Z. J., Small, 2015, 11(28), 3444
Guo R. S., Yu Y., Zeng J. F., Liu X. Q., Zhou X. C., Niu L. Y., Gao T. T., Li K., Yang Y., Zhou F., Zheng Z. J., Adv. Sci., 2015, 2(3)
Cheng Y., Wang R., Sun J., Gao L., ACS Nano, 2015, 9(4), 3887
Zhao Y., Dong D., Wang Y., Gong S., An T., Yap L. W., Cheng W., ACS Appl. Mater. Interfaces, 2018, 10(49), 42612
Woo J., Lee H., Yi C., Lee J., Won C., Oh S., Jekal J., Kwon C., Lee S., Song J., Choi B., Jang K. I., Lee T., Adv. Funct. Mater., 2020, 30(29), 1910026
Zhao Y., Tan Y. J., Yang W., Ling S., Yang Z., Teo J. T., See H. H., Lee D. K. H., Lu D., Li S., Zeng X., Liu Z., Tee B. C. K., Adv. Healthcare Mater., 2021, 10(17), 2100221
Kanik M., Orguc S., Varnavides G., Kim J., Benavides T., Gonzalez D., Akintilo T., Tasan C. C., Chandrakasan A. P., Fink Y., Anikeeva P., Science, 2019, 365(6449), 145
Cho Y., Shin J. H., Costa A., Kim T. A., Kunin V., Li J., Lee S. Y., Yang S., Han H. N., Choi I. S., Srolovitz D. J., Proc. Natl. Acad. Sci., 2014, 111(49), 17390
Blees M. K., Barnard A. W., Rose P. A., Roberts S. P., McGill K. L., Huang P. Y., Ruyack A. R., Kevek J. W., Kobrin B., Muller D. A., McEuen P. L., Nature, 2015, 524(7564), 204
Shyu T. C., Damasceno P. F., Dodd P. M., Lamoureux A., Xu L., Shlian M., Shtein M., Glotzer S. C., Kotov N. A., Nat. Mater., 2015, 14(8), 785
Zhang Y., Yan Z., Nan K., **ao D., Liu Y., Luan H., Fu H., Wang X., Yang Q., Wang J., Ren W., Si H., Liu F., Yang L., Li H., Wang J., Guo X., Luo H., Wang L., Huang Y., Rogers J. A., Proc. Natl. Acad. Sci., 2015, 112(38), 11757
Rafsanjani A., Bertoldi K., Phys. Rev. Lett., 2017, 118(8), 084301
Wang Z. H., Zhang L., Duan S. S., Jiang H., Shen J. H., Li C. Z., J. Mater. Chem. C, 2017, 5(34), 8714
Brooks A. K., Chakravarty S., Ali M., Yadavalli V. K., Adv. Mater., 2022, 34, 2109550
Li X., Zhu P., Zhang S., Wang X., Luo X., Leng Z., Zhou H., Pan Z., Mao Y., ACS Nano, 2022, 16, 5909
Pradhan S., Ventura L., Agostinacchio F., Xu M., Barbieri E., Motta A., Pugno N. M., Yadavalli V. K., ACS Appl. Mater. Interfaces, 2020, 12(11), 12436
Won P., Park J. J., Lee T., Ha I., Han S., Choi M., Lee J., Hong S., Cho K. J., Ko S. H., Nano Lett., 2019, 19(9), 6087
Morikawa Y., Yamagiwa S., Sawahata H., Numano R., Koida K., Kawano T., Adv. Healthcare Mater., 2019, 8(23), 1900939
Xu R., Zverev A., Hung A., Shen C., Irie L., Ding G., Whitmeyer M., Ren L., Griffin B., Melcher J., Zheng L., Zang X., Sanghadasa M., Lin L., Microsyst. Nanoeng., 2018, 4, 36
Morikawa Y., Yamagiwa S., Sawahata H., Numano R., Koida K., Ishida M., Kawano T., Adv. Healthcare Mater., 2018, 7(3), 1701100
Guan Y. S., Zhang Z. L., Tang Y. C., Yin J., Ren S. Q., Adv. Mater., 2018, 30(20), 1706390
Lv Z., Luo Y., Tang Y., Wei J., Zhu Z., Zhou X., Li W., Zeng Y., Zhang W., Zhang Y., Qi D., Pan S., Loh X. J., Chen X., Adv. Mater., 2018, 30(2), 1704531
Jung D., Lim C., Shim H. J., Kim Y., Park C., Jung J., Han S. I., Sunwoo S. H., Cho K. W., Cha G. D., Kim D. C., Koo J. H., Kim J. H., Hyeon T., Kim D. H., Science, 2021, 373(6558), 1022
Guo F., Jiang Y., Xu Z., **ao Y., Fang B., Liu Y., Gao W., Zhao P., Wang H., Gao C., Nat. Commun., 2018, 9(1), 881
Liu Z., Yu M., Lv J., Li Y., Yu Z., ACS Appl. Mater. Interfaces, 2014, 6(16), 13487
Lacour S. P., Chan D., Wagner S., Li T., Suo Z., Appl. Phys. Lett., 2006, 88(20), 204103
Graudejus O., Jia Z., Li T., Wagner S., Scr. Mater., 2012, 66(11), 919
Chen G., Matsuhisa N., Liu Z., Qi D., Cai P., Jiang Y., Wan C., Cui Y., Leow W. R., Liu Z., Gong S., Zhang K. Q., Cheng Y., Chen X., Adv. Mater., 2018, 30(21), 1800129
Yan X., Liu Z., Zhang Q., Lopez J., Wang H., Wu H.-C., Niu S., Yan H., Wang S., Lei T., Li J., Qi D., Huang P., Huang J., Zhang Y., Wang Y., Li G., Tok J. B. H., Chen X., Bao Z., J. Am. Chem. Soc., 2018, 140(15), 5280
Lee S. Y., Park K. R., Kang S. G., Lee J. H., Jeon E. C., Shim C. H., Ahn J. P., Kim D. I., Han H. N., Joo Y. C., Kim C., Choi I. S., Nat. Commun., 2019, 10(1), 4454
Matsuhisa N., Jiang Y., Liu Z. Y., Chen G., Wan C. J., Kim Y., Kang J., Tran H., Wu H. C., You I., Bao Z. A., Chen X. D., Adv. Electron. Mater., 2019, 5(8), 1900347
Hong S., Lee H., Lee J., Kwon J., Han S., Suh Y. D., Cho H., Shin J., Yeo J., Ko S. H., Adv. Mater., 2015, 27(32), 4744
Jiang Z., Nayeem M. O. G., Fukuda K., Ding S., ** H., Yokota T., Inoue D., Hashizume D., Someya T., Adv. Mater., 2019, 31(37), 1903446
Lipomi D. J., Vosgueritchian M., Tee B. C. K., Hellstrom S. L., Lee J. A., Fox C. H., Bao Z. N., Nat. Nanotechnol., 2011, 6(12), 788
Xu F., Zhu Y., Adv. Mater., 2012, 24(37), 5117
Kim D. H., Yu K. C., Kim Y., Kim J. W., ACS Appl. Mater. Interfaces, 2015, 7(28), 15214
Wang T., Wang R. R., Cheng Y., Sun J., ACS Appl. Mater. Interfaces, 2016, 8(14), 9297
Xu F., Wang X., Zhu Y. T., Zhu Y., Adv. Electron. Mater., 2012, 22(6), 1279
** Y., Hwang S., Ha H., Park H., Kang S. W., Hyun S., Jeon S., Jeong S. H., Adv. Electron. Mater., 2016, 2(2), 1500302
Li P., Zhang W., Ma J. G., Wang X., Xu H. Y., Cong L. J., Liu Y. C., Adv. Electron. Mater., 2018, 4(12), 1800346
Won Y., Kim A., Yang W., Jeong S., Moon J., NPG Asia Mater., 2014, 6, e132
Jang N. S., Kim K. H., Ha S. H., Jung S. H., Lee H. M., Kim J. M., ACS Appl Mater Interfaces, 2017, 9(23), 19612
Song P., Qin H. L., Gao H. L., Cong H. P., Yu S. H., Nat. Commun., 2018, 9, 2786
Xue J., Zou Y., Deng Y., Li Z., EcoMat, 2022, e12209
Lee J., Leung V., Lee A.-H., Huang J., Asbeck P., Mercier P. P., Shellhammer S., Larson L., Laiwalla F., Nurmikko A., Nat. Electron., 2021, 4(8), 604
Donega M., Fjordbakk C. T., Kirk J., Sokal D. M., Gupta I., Hunsberger G. E., Crawford A., Cook S., Viscasillas J., Stathopoulou T. R., Miranda J. A., Dopson W. J., Goodwin D., Rowles A., McGill P., McSloy A., Werling D., Witherington J., Chew D. J., Perkins J. D., Proc. Natl. Acad. Sci. USA, 2021, 118(20), e2025428118
**e L. S., Skorupskii G., Dinca M., Chem. Rev., 2020, 120(16), 8536
Gao L.-L., Gao E.-Q., Coord. Chem. Rev., 2021, 434, 213784
Li J., Liu Y., Yuan L., Zhang B., Bishop E. S., Wang K., Tang J., Zheng Y. Q., Xu W., Niu S., Beker L., Li T. L., Chen G., Diyaolu M., Thomas A. L., Mottini V., Tok J. B., Dunn J. C. Y., Cui B., Pasca S. P., Cui Y., Habtezion A., Chen X., Bao Z., Nature, 2022, 606(7912), 94
Dickey M. D., Adv. Mater., 2017, 29(27), 1606425
Ma Z. J., Huang Q. Y., Xu Q., Zhuang Q. N., Zhao X., Yang Y. H., Qiu H., Yang Z. L., Wang C., Chai Y., Zheng Z. J., Nat. Mater., 2021, 20(6), 859
Liu S. Z., Shah D. S., Kramer-Bottiglio R., Nat. Mater., 2021, 20(6), 851
Leber A., Dong C., Chandran R., Das Gupta T., Bartolomei N., Sorin F., Nat. Electron., 2020, 3(6), 316
Cao J., Liang F., Li H., Li X., Fan Y., Hu C., Yu J., Xu J., Yin Y., Li F., Xu D., Feng H., Yang H., Liu Y., Chen X., Zhu G., Li R. W., InfoMat, 2022, 4(4), e12302
Park J. E., Kang H. S., Koo M., Park C., Adv. Mater., 2020, 32(37), 2002178
Hwang H., Kong M., Kim K., Park D., Lee S., Park S., Song H.-J., Jeong U., Sci. Adv., 2021, 7(32), eabh0171
Zhu M., Ji S., Luo Y., Zhang F., Liu Z., Wang C., Lv Z., Jiang Y., Wang M., Cui Z., Li G., Jiang L., Liu Z., Chen X., Adv. Mater., 2022, 34, e2101339
Li W., Matsuhisa N., Liu Z., Wang M., Luo Y., Cai P., Chen G., Zhang F., Li C., Liu Z., Lv Z., Zhang W., Chen X., Nat. Electron., 2021, 4(2), 134
Luo Y., Li W., Lin Q., Zhang F., He K., Yang D., Loh X. J., Chen X., Adv. Mater., 2021, 33(14), 200784
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This work was supported by the National Research Foundation(NRF), Prime Minister’s Office, Singapore, under NRF Investigatorship(NRF-NRFI2017-07), A*STAR Advanced Manufacturing and Engineering(AME) Programmatic Grant (No.A18A1b0045).
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Zhang, F., Chen, X. Bioinspired Strategies for Stretchable Conductors. Chem. Res. Chin. Univ. 39, 30–41 (2023). https://doi.org/10.1007/s40242-022-2236-1
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DOI: https://doi.org/10.1007/s40242-022-2236-1