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Article
Open AccessMultiphoton Phosphorescence of Simple Ketones by Visible-light Excitation and Its Consideration for Active Sensing in Space
Acetone and butanone were seen to emit blue light around 450 nm when excited in the green by a high intensity pulsed laser. The pathway of this anti-Stokes emission is believed to be multiphoton absorption fol...
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Article
Endothermic singlet fission is hindered by excimer formation
Singlet fission is a process whereby two triplet excitons can be produced from one photon, potentially increasing the efficiency of photovoltaic devices. Endothermic singlet fission is desired for a maximum en...
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Article
Open AccessAcoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast o...
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Article
Vibrational coherence probes the mechanism of ultrafast electron transfer in polymer–fullerene blends
The conversion of photoexcitations into charge carriers in organic solar cells is facilitated by the dissociation of excitons at the donor/acceptor interface. The ultrafast timescale of charge separation deman...
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Chapter and Conference Paper
Femtosecond multicolor pump-probe investigation of ultrafast electron transfer of (NH3)5RuIIINCRuII(CN)5 - in solution
Ultrafast measurements on (NH3)5RuIIINCRuII(CN)5 - in solution reveal an ultrafast spectral component due to vibrationally unrelaxed stimulated emission, allowing for new insights on the interplay...