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Article
Single-shot pulse duration monitor for extreme ultraviolet and X-ray free-electron lasers
The resolution of ultrafast studies performed at extreme ultraviolet and X-ray free-electron lasers is still limited by shot-to-shot variations of the temporal pulse characteristics. Here we show a versatile s...
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Article
High-Field DNP Spectrometer for Liquids
The construction of a prototype 400 MHz/260 GHz (9.2 T) liquid-state dynamic nuclear polarization (DNP) spectrometer is described. For this purpose a 400 MHz Bruker Avance nuclear magnetic resonance spectromet...
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Article
Open AccessFirst DNP Results from a Liquid Water-TEMPOL Sample at 400 MHz and 260 GHz
Using a newly designed liquid-state dynamic nuclear polarization (DNP) spectrometer operating at a magnetic field of 9.2 T, a DNP enhancement of −4.0(1) was achieved for protons in a liquid water-TEMPOL sample...
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Article
Investigations of “soft-landed” Cd surface atoms via nuclear methods: hyperfine-field sign determination
Using refined preparation techniques, cadmium guest atoms have been positioned at different sites on the surfaces of nickel crystals. The magnetic hyperfine fields and the electric field gradients at the Cd ...
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Article
Magnetic anisotropy of Ni modified by extreme lattice expansion
The induced magnetism of isolated (Cd) adatoms, soft-landed onto ultrathin Ni layers grown pseudo-morphologically on Pd(001) (aPd = 3.8907 Å), was studied using the perturbed angular correlation (PAC) technique. ...
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Article
A study of the induced magnetism in the Au spacer layer of Co/Au/CoO exchange-bias trilayers and related systems
We report the first observation of the effects of exchange bias on the nuclear spin polarization and induced magnetic moments at a magnetic/non-magnetic interface, applying low temperature nuclear orientation (LT...
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Chapter and Conference Paper
Surface and Interface Magnetism Using Radioactive Probes
Magnetic properties of impurities at ferromagnetic surfaces and interfaces have been investigated performing Perturbed Angular Correlation (PAC) measurements in the ultra-high vacuum chamber ASPIC (Apparatus f...
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Article
Surface and Interface Magnetism Using Radioactive Probes
Magnetic properties of impurities at ferromagnetic surfaces and interfaces have been investigated performing Perturbed Angular Correlation (PAC) measurements in the ultra-high vacuum chamber ASPIC (Apparatus f...
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Article
Observation of magnetization rotation during the reversal in Co/CoO exchange-bias multilayers
The magnetization-reversal processes of ferromagnetic Co in [Co/CoO/Au]20 exchange-bias multilayers are studied with polarized neutron reflectometry. The investigations were performed at 300 K, i.e. above the Née...
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Article
Step-induced canting of magnetization in Fe/Ag superlattices
We have investigated the reorientation of the easy axis of magnetization in (0 0 1) Fe/Ag superlattices using vibrating sample magnetometry, Mössbauer spectroscopy and nuclear resonance scattering of synchrotr...
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Article
A study of the induced magnetic hyperfine fields in Fe/Ag multilayers
Near perpendicular magnetic hyperfine fields in 110mAg have been observed in Fe/Ag multilayers. These fields are studied by low temperature nuclear orientation (LTNO) in multilayers [Ag(x ML)/Fe(y ML)]20, with (x...
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Article
A low temperature study of antiferromagnetic YbVO4 by NMR thermally detected by nuclear orientation
NMR-TDNO results using an external 60CoCo (hcp) nuclear orientation thermometer for non-irradiated, single crystal, antiferromagnetic YbVO4 are compared with those obtained earlier with neutron activated samples ...
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Article
NMRON studies of MnBr2 \(\cdot \) 4H2O in applied magnetic fields
NMRON studies for the \(\left. {| \pm 3} \right\rangle \to \left. {| \pm 2} \right\rangle \) 54Mn transitions in an...
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Article
Some analytical results forABC, ABCD, andXBCD coupled spin 1/2 systems. II
In the preceding paper, it was shown that the calculation of the density matrixρ(t) for multiply connectedABC, etc., spin 1/2 spin systems can be greatly simplified by subdividing the Hamiltonian ...
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Article
Some analytical results for spin 1/2 spin systems. III: The benzene ring
In two earlier papers on multiply connectedABCD spin 1/2 spin systems, it was shown that it is possible to simplify the calculation of (i) the time dependent density matrixϱ(t), and (ii) the time evolution of hig...
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Article
A nuclear orientation study of YbVO4
Nuclear orientation studies on single crystals of tetragonal YbVO4 are reported, using the radioactive isotopes169Yb (I=7/2), and175Yb (I=7/2). The anisotropies for a number of gamma-rays of both isotopes have be...
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Article
Irreducible half-integer rank unit spherical tensors
A new class of half-integer rank spherical tensors is introduced. The motivation for investigating this new class of tensors originated from a desire to be able to partition matrices using mixtures of fictitio...
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Article
Complete solution for two coupled spin-1/2 nuclei evolving under chemical shift and dipolar interaction
The spin dynamics for two coupled spin-1/2 nuclei evolving under isotropic chemical shifts and a dipole-dipole interaction, in the high-field limit, is presented using Fano's unit spherical tensors ...
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Article
Analytical block-diagonalization of matrices using unit spherical tensors
A new method for block-diagonalizing large Hamiltonian matrices, in closed form, is described. The method is based on (i) a general unitary transformation due to Slichter, and (ii) Fano's unit spherical operators