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A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy
Electrification to reduce or eliminate greenhouse gas emissions is essential to mitigate climate change. However, a substantial portion of our manufacturing and transportation infrastructure will be difficult ...
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Article
Biorenewable and circular polydiketoenamine plastics
Amid growing concerns over the human health and environmental impacts of plastic waste, the most promising solution would be to build a circular plastics economy where sustainability considerations dictate the...
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Article
Electrifying the upcycling of plastics
Polyvinyl chloride (PVC) is challenging to recycle owing to the formation of hydrochloric acid during depolymerization at high temperatures. Now, a method for upcycling PVC that relies on its intrinsic reactiv...
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Article
Continuous, autonomous subsurface cargo shuttling by nature-inspired meniscus-climbing systems
Water-walking insects can harness capillary forces by changing their body posture to climb or descend the meniscus between the surface of water and a solid object. Controlling surface tension in this manner is...
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Article
Diversity-oriented synthesis of polymer membranes with ion solvation cages
Microporous polymers feature shape-persistent free volume elements (FVEs), which are permeated by small molecules and ions when used as membranes for chemical separations, water purification, fuel cells and ba...
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Universal chemomechanical design rules for solid-ion conductors to prevent dendrite formation in lithium metal batteries
Dendrite formation during electrodeposition while charging lithium metal batteries compromises their safety. Although high-shear-modulus (Gs) solid-ion conductors (SICs) have been prioritized to resolve the press...
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Article
Closed-loop recycling of plastics enabled by dynamic covalent diketoenamine bonds
Recycled plastics are low-value commodities due to residual impurities and the degradation of polymer properties with each cycle of re-use. Plastics that undergo reversible polymerization allow high-value mono...
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Open AccessHarnessing liquid-in-liquid printing and micropatterned substrates to fabricate 3-dimensional all-liquid fluidic devices
Systems comprised of immiscible liquids held in non-equilibrium shapes by the interfacial assembly and jamming of nanoparticle−polymer surfactants have significant potential to advance catalysis, chemical sepa...
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Open AccessMolecular understanding of polyelectrolyte binders that actively regulate ion transport in sulfur cathodes
Polymer binders in battery electrodes may be either active or passive. This distinction depends on whether the polymer influences charge or mass transport in the electrode. Although it is desirable to understa...
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Bicontinuous structured liquids with sub-micrometre domains using nanoparticle surfactants
Polymer–nanoparticle binding stabilizes bijels with sub-micrometre domain size.
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Article
IDEAL: Images Across Domains, Experiments, Algorithms and Learning
Research across science domains is increasingly reliant on image-centric data. Software tools are in high demand to uncover relevant, but hidden, information in digital images, such as those coming from faster...
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Correction: Corrigendum: H+-type and OH−-type biological protonic semiconductors and complementary devices
Proton conduction is essential in biological systems. Oxidative phosphorylation in mitochondria, proton pum** in bacteriorhodopsin, and uncoupling membrane potentials by the antibiotic Gramicidin are example...
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Article
Enhanced thermal transport at covalently functionalized carbon nanotube array interfaces
It has been more than a decade since the experimental demonstration that the thermal conductivity of carbon nanotubes can exceed that of diamond, which has the highest thermal conductivity among naturally occu...
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Erratum: H+-type and OH−-type biological protonic semiconductors and complementary devices
Scientific Reports 3, Article number: 2481 (2013); Published: 3 October 2013; Updated: 1 November 2013 The incorrect version of the Supplementary Information file was inadvertently published with this Article....
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Open AccessH+-type and OH−-type biological protonic semiconductors and complementary devices
Proton conduction is essential in biological systems. Oxidative phosphorylation in mitochondria, proton pum** in bacteriorhodopsin and uncoupling membrane potentials by the antibiotic Gramicidin are examples...