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Book
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Book
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Book
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Book
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Book
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Book
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Book
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Chapter
Phases and Phase Changes of Small Systems
Atomic and molecular clusters exhibit a variety of phase-like forms and phase changes that differ from those of bulk matter. It is possible to relate some-but not all-of these to corresponding phases and phase...
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Article
Size is everything
Bulk matter melts and freezes in a predictable manner. Not so clusters of atoms in their tens, hundreds or thousands, which have very different properties. They have no fixed melting temperature at a given pre...
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Book
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Article
Thermal Mass and Thermal Inertia in Fluids — A Comparison of Hypotheses
Thermal inertia and thermal mass are concepts that offer means to describe transport of heat in nonequilibrium fluids. However there are options regarding how to separate the part of the total flow that caries...
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Chapter
Phases and Phase Changes of Clusters
Phase-like forms are expected to be observable for many kinds of clusters, insofar as they should satisfy criteria used to characterize phases of bulk form. However clusters are also expected to exhibit phase-...
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Chapter
Topographies and Dynamics of Many-Dimensional Potential Surfaces
Multidimensional potential surfaces pose a variety of problems, not least of which is that it is now possible to obtain more information about the minima and other stationary points of such surfaces than we kn...
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Chapter
Probing The Collective and Independent-Particle Character of Atomic Electrons
Niels Bohr and Arnold Sommerfeld developed their model of the hydrogen atom and other one-electron atoms based on the concepts of discrete, stationary states and quantized energies and angular momenta of these...
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Chapter
Exploring Potential Surface Landscapes and How they Govern Dynamics
The subject of multidimensional potential surfaces and the dynamics on those surfaces was just reviewed by this writer 1, and the closely related topic of the analytic representation of potential surfaces, largel...
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Chapter
Phase Transitions in Clusters: A Bridge to Condensed Matter
Clusters of atoms or molecules, consisting of as few as three and as many as many thousands of particles, exhibit some properties of individual molecules, some properties of bulk matter and some properties cha...
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Article
Preface
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Article
Chaotic dynamics and vibrational mode coupling in small argon clusters
We have computed the local Kolmogorov entropy of molecular dynamics trajectory segments near the potential energy saddles of model Ar3 and Ar5 clusters. In the case of Ar3 clusters bound with a Lennard-Jones pote...
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Article
Clusters: A laboratory for studying chaos and ergodicity
The dynamics of clusters are revealed, in part, by the extent and nature of their chaotic and ergodic behavior. Conversely, small clusters offer opportunities to study the origins and evolution of chaotic and ...
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Article
Noble gas clusters in model zeolite cavities
Noble gas atoms trapped in the intracrystalline cavities of zeolites may form clusters. A classical-mechanical isoenergetic molecular dynamics simulation is performed to simulate the dynamical behavior of nobl...