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  1. No Access

    Article

    Mono-, Bi- and Multifunctional Single-Sites: Exploring the Interface Between Heterogeneous and Homogeneous Catalysis

    This mini-review contrasts the characteristics of traditional heterogeneous (solid) catalysts with those of homogeneous ones: the nature of the active sites in each case is very different, a fact well illustra...

    John Meurig Thomas, Robert Raja in Topics in Catalysis (2010)

  2. No Access

    Article

    Single-site Biomimetic Amino Acid Complexes for the Benign Oxidation of Hydrocarbons and Alcohols

    Zeolite encapsulated amino acid complexes such as Fe-proline, Fe-histidine and Cu-valine have shown significant promise in the selective oxidation of hydrocarbons such as cyclohexane and benzylic alcohols. Thi...

    Joanna Dzierzak, Michael Lefenfeld, Robert Raja in Topics in Catalysis (2009)

  3. No Access

    Article

    Designed Nanoporous Solids for the Green Production of Vitamins, Fine Chemicals and Renewable Nylons

    Designed nanoporous solids are highly effective in facilitating shape-selective and regiospecific catalytic conversions in the synthesis of fine chemicals, pharmaceutical intermediates as well as in sustainabl...

    Robert Raja in Topics in Catalysis (2009)

  4. No Access

    Article

    The advantages and future potential of single-site heterogeneous catalysts

    Using open-structure (nanoporous) solids, advantage may be taken of single-site catalytically active centres to effect an enormous range of conversions of organic compounds where regio-selectivity and shape-se...

    John Meurig Thomas, Robert Raja in Topics in Catalysis (2006)

  5. No Access

    Article

    A New Approach to the Design of Heterogeneous Single-Site Enantioselective Catalysts

    We analyze the merits of an approach to the design of enantioselective catalysts that relies on constraining an anchored organometallic complex at the inner walls of mesoporous silica. Two distinct metal cente...

    Matthew D. Jones, Robert Raja, John Meurig Thomas… in Topics in Catalysis (2003)

  6. No Access

    Article

    Towards an Environmentally Acceptable Heterogeneous Catalytic Method of Producing Adipic Acid by the Oxidation of Hydrocarbons in Air

    A survey is given of the catalytic methods potentially available for the production of adipic acid by the oxidation of readily available hydrocarbon precursors under environmentally benign conditions. Encourag...

    Robert Raja, Sang-Ok Lee, Manuel Sanchez-Sanchez, Gopinathan Sankar… in Topics in Catalysis (2002)