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Clarifying the relationship between redox activity and electrochemical stability in solid electrolytes

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    Thermodynamics of multi-sublattice battery active materials: from an extended regular solution theory to a phase-field model of LiMnyFe1-yPO4

    Phase separation during the lithiation of redox-active materials is a critical factor affecting battery performance, including energy density, charging rates, and cycle life. Accurate physical descriptions of ...

    Pierfrancesco Ombrini, Martin Z. Bazant, Marnix Wagemaker… in npj Computational Materials (2023)

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