Abstract
This work is focused on the analysis of the quantum dynamics of a model one-dimensional lattice array of quantum dots on a two dimensional electron sheet/layer in a normal magnetic field. Our analysis is carried out with the derivation of the Green’s function for the quantum dot lattice subject to Landau quantization using the corresponding “no-lattice” Green’s function, for propagation along the axis of the 1D quantum dot lattice. The frequency/energy poles of this Green’s function provide the dispersion relation for the Landau quantized energy spectrum, which exhibits Landau minibands, rather than discrete Landau levels. In the case of nonrelativistic carriers, the dispersion relation is explicitly exhibited in a closed form in terms of the Jacobi Theta Function of the third kind, and an approximate solution displaying the Landau miniband formation is obtained in terms of Laguerre polynomials. We also examine the case of “relativistic” graphene carriers, employing the appropriate Landau quantized graphene Green’s function in a study of the associated wave packet dynamics in a graphene antidot lattice in a normal magnetic field. In this, we analyze the effects of pseudospin on the wave packet dynamics in Landau quantized graphene, including the role of Zitterbewegung in circular orbit motion.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Similar content being viewed by others
References
L.L. Sohn, L.P. Kouwenhoven, G. Schoen, Mesoscopic Electron Transport (Springer and Kluwer, Netherlands, 1997)
C.R. Kagan, C.B. Murray, Charge transport in strongly coupled quantum dot solids. Nat. Nanotechnol. 10(12), 1013–1026 (2015)
V.P. Kunets, M. Rebello Sousa Dias, T. Rembert, M.E. Ware, Y.I. Mazur, V. Lopez-Richard, H.A. Mantooth, G.E. Marques, G.J. Salamo, Electron transport in quantum dot chains: dimensionality effects and hop** conductance. J. Appl. Phys. 113(18), 183709 (2013)
T. Jamieson, R. Bakhshi, D. Petrova, R. Pocock, M. Imani, A.M. Seifalian, Biological applications of quantum dots. Biomaterials 28(31), 4717–4732 (2007)
L. Qi, X. Gao, Emerging application of quantum dots for drug delivery and therapy. Expert Opin. Drug Deliv. 5(3), 263–267 (2008). (PMID: 18318649)
National Research Council, High Magnetic Field Science and Its Application in the United States: Current Status and Future Directions (The National Academies Press, Washington, D.C., 2013)
D. Lai, Matter in strong magnetic fields. Rev. Mod. Phys. 73, 629–662 (2001)
N.J.M. Horing, S. Bahrami, Landau minibands in an antidot lattice. AdvNanoBio M & D 1(1), 24 (2017)
N.J. Morgenstern Horing, S.Y. Liu, Green’s functions for a graphene sheet and quantum dot in a normal magnetic field. J. Phys. A: Math. Theor. 42(22), 225301 (2009)
** Chen, V.I. Fal’ko, Hierarchy of gaps and magnetic minibands in graphene in the presence of the Abrikosov vortex lattice. Phys. Rev. B 93, 035427 (2016)
C. Kittel. Introduction to Solid State Physics, 7th edn. (Wiley, 1991)
N.J. Morgenstern Horing, M.M. Yildiz, Quantum theory of longitudinal dielectric response properties of a two-dimensional plasma in a magnetic field. Ann. Phys. 97(1), 216–241 (1976)
A. Erdelyi, H. Bateman, Higher Transcendental Functions, vol. 2 (McGraw-Hill, 1953)
T. Ando, Theory of electronic states and transport in carbon nanotubes. J. Phys. Soc. Jpn. 74(3), 777–817 (2005)
Y. Zheng, T. Ando, Hall conductivity of a two-dimensional graphite system. Phys. Rev. B 65, 245420 (2002)
N.J.M. Horing, Landau quantized dynamics and spectra for group-vi dichalcogenides, including a model quantum wire. AIP Adv. 7(6), 065316 (2017)
N.J.M. Horing, Addendum: “Landau quantized dynamics and spectra for group-vi dichalcogenides, including a model quantum wire” [AIP Advances 7, 065316 (2017)]. AIP Adv. 8(4), 049901 (2018)
Q. Wang, R. Shen, L. Sheng, B.G. Wang, D.Y. **ng, Transient zitterbewegung of graphene superlattices. Phys. Rev. A 89, 022121 (2014)
G.M. Maksimova, V.Y. Demikhovskii, E.V. Frolova, Wave packet dynamics in a monolayer graphene. Phys. Rev. B 78, 235321 (2008)
V.Y. Demikhovskii, G.M. Maksimova, E.V. Frolova, Wave packet dynamics in a two-dimensional electron gas with spin orbit coupling: Splitting and zitterbewegung. Phys. Rev. B 78, 115401 (2008)
R.A.W. Ayyubi, N.J.M. Horing, K. Sabeeh, Effect of pseudospin polarization on wave packet dynamics in graphene antidot lattices (gals) in the presence of a normal magnetic field. J. Appl. Phys. 129(7), 074301 (2021)
D. Song, V. Paltoglou, S. Liu, Y. Zhu, D. Gallardo, L. Tang, J. Xu, M. Ablowitz, N.K. Efremidis, Z. Chen, Unveiling pseudospin and angular momentum in photonic graphene. Nat. Commun. 6, 6272 (2015)
Tomasz M. Rusin, Wlodek Zawadzki, Zitterbewegung of electrons in graphene in a magnetic field. Phys. Rev. B 78, 125419 (2008)
E. Serna, I. Rodríguez Vargas, R. Pérez-Álvarez, L. Diago-Cisneros, Pseudospin-dependent zitterbewegung in monolayer graphene. J. Appl. Phys. 125(20), 203902 (2019)
L. Esaki, R. Tsu, Superlattice and negative differential conductivity in semiconductors. IBM J. Res. Dev. 14(1), 61–65 (1970)
C. Heide, T. Higuchi, H.B. Weber, P. Hommelhoff, Coherent electron trajectory control in graphene. Phys. Rev. Lett. 121, 207401 (2018)
A.H. Castro Neto, F. Guinea, N.M.R. Peres, K.S. Novoselov, A.K. Geim, The electronic properties of graphene. Rev. Mod. Phys. 81, 109–162 (2009)
C.H. Park, Y.W. Son, L. Yang, M.L. Cohen, S.G. Louie, Electron beam supercollimation in graphene superlattices. Nano Lett. 8(9), 2920 (2008)
S. Choi, C.-H. Park, S.G. Louie, Electron supercollimation in graphene and Dirac fermion materials using one-dimensional disorder potentials. Phys. Rev. Lett. 113, 026802 (2014)
C.-H. Park, L. Yang, Y.-W. Son, M.L. Cohen, S.G. Louie, Anisotropic behaviours of massless Dirac fermions in graphene under periodic potentials (2008)
T.G. Pedersen, C. Flindt, J. Pedersen, N.A. Mortensen, A.-P. Jauho, K. Pedersen, Graphene antidot lattices: designed defects and spin qubits. Phys. Rev. Lett. 100, 136804 (2008)
A.J.M. Giesbers, E.C. Peters, M. Burghard, K. Kern, Charge transport gap in graphene antidot lattices. Phys. Rev. B 86, 045445 (2012)
N.J. Morgenstern Horing, Dichalcogenide Landau miniband dynamics and spectrum in an antidot superlattice. AIP Adv. 10(3), 035203 (2020)
T. Danz, A. Neff, J.H. Gaida, R. Bormann, C. Ropers, S. Schäfer, Ultrafast sublattice pseudospin relaxation in graphene probed by polarization-resolved photoluminescence. Phys. Rev. B 95, 241412 (2017)
S. Aeschlimann, R. Krause, M. Chávez-Cervantes, H. Bromberger, R. Jago, E. Malić, A. Al-Temimy, C. Coletti, A. Cavalleri, I. Gierz, Ultrafast momentum imaging of pseudospin-flip excitations in graphene. Phys. Rev. B 96, 020301 (2017)
M. Trushin, A. Grupp, G. Soavi, A. Budweg, D. De Fazio, U. Sassi, A. Lombardo, A.C. Ferrari, W. Belzig, A. Leitenstorfer, D. Brida, Ultrafast pseudospin dynamics in graphene. Phys. Rev. B 92, 165429 (2015)
Chen-Di Han, Hong-Ya Xu, Ying-Cheng Lai, Pseudospin modulation in coupled graphene systems. Phys. Rev. Research 2, 033406 (2020)
M. Polini, F. Guinea, M. Lewenstein, H. Manoharan, V. Pellegrini, Artificial honeycomb lattices for electrons, atoms and photons. Nat. Nanotechnol. 8, 625–633 (2013)
K. Gomes, W. Mar, W. Ko, F. Guinea, H. Manoharan, Designer Dirac fermions and topological phases in molecular graphene. Nature 483, 306–310 (2012)
O. Bahat-Treidel, O. Peleg, M. Grobman, N. Shapira, M. Segev, T. Pereg-Barnea, Klein tunneling in deformed honeycomb lattices. Phys. Rev. Lett. 104, 063901 (2010)
P. Soltan-Panahi, J. Struck, P. Hauke, A. Bick, W. Plenkers, G. Meineke, C. Becker, P. Windpassinger, M. Lewenstein, K. Sengstock, Multi-component quantum gases in spin-dependent hexagonal lattices. Nat. Phys. 7, 05 (2010)
Tomasz M. Rusin, Wlodek Zawadzki, Transient zitterbewegung of charge carriers in mono- and bilayer graphene, and carbon nanotubes. Phys. Rev. B 76, 195439 (2007)
A.O. Barut, A.J. Bracken, Zitterbewegung and the internal geometry of the electron. Phys. Rev. D 23, 2454–2463 (1981)
F. Schwabl, Advanced Quantum Mechanics, 4th edn. (Springer, Berlin, 2008)
Acknowledgement
This chapter replicates some work presented in our earlier publication “Landau Minibands in an Antidot Lattice” in AdvNanoBio M & D 1 (1), 24 (2017) [8]. The appearance of the work in this chapter is facilitated by the gracious consent of the journal editor, Prof. Dr. Anton Ficai of SciEdTech.eu.
Author information
Authors and Affiliations
Corresponding author
Editor information
Editors and Affiliations
Appendices
Appendix A
16.11 Zitterbewegung Phenomenon
Zitterbewegung is the jittery motion of the Dirac electron. It occurs when one tries to confine the Dirac electrons. According to the Heisenberg uncertainty principle, localization of the electron wave packet leads to uncertainty in momentum. For particles with zero rest mass (massless Dirac particles), uncertainty in momentum translates into uncertainty in energy of the particle (This should be contrasted with the nonrelativistic case, where the position-momentum uncertainty relation is independent of the energy-time uncertainty relation) [27].
16.1.1 16.11.1 Prediction and Interpretation of Zitterbewegung by Schrödinger
Schrödinger discovered a highly oscillatory motion of the electron with velocity c during his work on the time evolution of the position operator, which he named Zitterbewegung [43]. Schrödinger attempted to explain this phenomenon in terms of microscopic dynamical variables i.e coordinate and momentum. To determine the time evolution of the position operator, Schrödinger used Dirac’s Hamiltonian for the free electron-positron system, which is
In the above equation \(\mathbf {\alpha }\) and \(\beta \) satisfy the following anti-commutation relations:
where \(i,j=1,2,3\) and I is a unit matrix. Also the momentum operator \(\textbf{q}\) and coordinate operator \(\textbf{x}\) commute with \(\mathbf {\alpha }\) and \(\beta \), and satisfy the canonical anti-commutation relations for Fermions
In the Heisenberg picture, the time derivative of any one of these operators, say A, which does not have explicit time dependence is given by
As a result
and (16.77) and (16.78) for the operator \(\mathbf {\alpha }\) give
Above equation can be written as
where we have defined
Schrödinger noted that
which yields
Using \(\{H,\mathbf {\eta }\}=0=\{H,\mathbf {\eta }_0\}\), (16.82) can also be written as
Combining (16.80), (16.81) and (16.83), Schrödinger obtained
which on integration yields
where \(\textbf{a}\) is an operator which is a constant of integration with the definition
Defining
equation (16.84) will become
where we have defined
Here, the term \(\mathbf {\xi } (t)\) corresponds to a microscopic coordinate which oscillates at high frequency known as Zitterbewegung (ZB). This motion is superimposed on a macroscopic type of motion associated with the coordinate \(\textbf{x}_A\). Characteristic amplitude associated with Zitterbewegung is \(\frac{\hbar }{2mc}\) and this amplitude is equal to half of the Compton wavelength of an electron, while the characteristic angular frequency of the Zitterbewegung is \(\frac{2mc^2}{\hbar }\).
Schrödinger went on to note, that if the orbital-angular momentum \(\textbf{L}\) and spin vector \(\textbf{S}\) are introduced as
then both \(\textbf{L}\) and \(\textbf{S}\) alone are not constant but their sum \(\textbf{L} + \textbf{S}\) is a constant of the motion. Schrödinger found
and
where \(\textbf{S}_A\) and \(\textbf{L}_A\) are constants and the term \(\mathbf {\eta } (t) \times \textbf{q}\) is oscillatory. Finally he found that
This constant of the motion allowed Schrödinger to explain Zitterbewegung in terms of microscopic dynamical variables spin and orbital angular momentum [43].
16.1.2 16.11.2 Zitterbewegung: Interpretation in Terms of Interference Between Positive and Negative Energy States
It can be easily verified that (16.84) along with (16.82) and (16.85) can be written as
Also (16.80) can be brought to the form
and hence
Along with the initial term \(\textbf{x}(0)\) at \(t = 0\), (16.88) also carries two more terms, one of them is linear in time t and corresponds to group velocity, while the second term is oscillatory in nature and is known as Zitterbewegung. \(\mathbf {\alpha } - \frac{c \textbf{q}}{H}\) is an operator whose matrix elements are required to evaluate the average value \(\int \psi ^\dagger (0,\textbf{x}) \textbf{x}(t) \psi (0,\textbf{x}) d^3x\). Nonvanishing matrix elements of this operator only lie between states of the same momentum. Also from (16.89), the anticommutator only vanishes when the energies are of opposite sign. Hence it can be concluded that ZB is a consequence of interference between positive and negative energy states as predicted by relativistic quantum mechanics [44].
Appendix B
16.12 Contour Integration
To solve the second integral in (16.69), let us denote the integral by I [21]
(\(I_2\) is unit matrix of order 2) where
Note that in the above integral, each “no lattice” Green’s function has real poles at \(\eta \)=\(\pm \sqrt{n}\). These “no lattice” poles of the term
can be seen to cancel by re-expressing the “no lattice” Green’s functions \(\dot{\tilde{\mathcal {G}}}^0(p;0,0;\eta )\) and \(\tilde{\mathcal {G}}^0(p;x_2;\eta )\). For this purpose, by using (16.58) and (16.59), one can easily write \(\alpha \dot{\tilde{\mathcal {G}}}^0(p;0,0;\eta )\) matrix as
where we have defined (j corresponds to the index r in (16.58, 16.59))
and
with
and
Similarly, the \(\tilde{\mathcal {G}}^0(p;x_2;\eta )\) matrix can be written as
where we have defined
and
with
and
Note that in the above equations, n is a Landau index and m is a dummy index for the Landau levels; the maximum value of n and m is the same.
Finally substituting (16.92) and (16.93) in (16.91), the matrix \(T_1\) becomes
In the above expression, the real “no lattice” poles (\(\eta \)=\(\pm \sqrt{n}\)) cancel. The above expression can be solved numerically. In this computation, it is also necessary to address the poles of the actual lattice Green’s function, which are defined by the zeros of the denominator, \(det\left[ I_2-\alpha \dot{\tilde{\mathcal {G}}}^0(p;0,0;\eta )\right] =0\), and these roots depend on p (and are not spaced by integer multiples of \(\omega _g\)): These poles are treated using the line broadening discussion of Sect. 16.5.2. The resultant \(2 \times 2\) matrix with \(c_{ij}(\eta )\) (where \(i,j=1,2\)) as matrix elements can be written as (substituting \(q=pd\))
Note that the above integral can be numerically calculated by applying the trapezoidal rule in the limits \(-\pi \) to \(\pi \), while kee** the trapezoidal step equal to \(\frac{\pi }{10}\); this gives an accuracy up to five decimal points for each value of \(n^\prime \).
Putting (16.94) in (16.90), the integral I becomes
It can be seen that the “no lattice” poles of the second integral (p integral) in (16.90) have been removed; and the poles of the actual lattice Green’s function have been dealt with using the line broadening of Sect. 16.5.2, so the only remaining poles that we have to deal with now are the poles of the matrix \(\mathcal {G}^0(x_1,n^\prime d;\eta )\).
Using (16.67) and (16.68), the matrix \( \alpha \mathcal {G}^0(x_1,n^\prime d;\eta )\) can be written as
where \(\Upsilon \), \(\gamma _1\) and \(\gamma _2\) are defined in (16.74) and (16.75). Using the matrices \(Q(\eta )\) and \( \alpha \mathcal {G}^0(x_1,n^\prime d;\eta )\) in (16.95), and breaking the matrix into two matrices, we get
(The first and second matrices correspond to n=0 and \(n>0\) Landau minibands, respectively.) In the above expression
and
In (16.97), the first matrix has a pole at \(\eta \)=0, while the second matrix has poles at \(\eta \)=\(\pm \sqrt{n}\). We now use contour integration with the Jordan lemma (closing the contour in the lower half plane for \(t>0\)) to evaluate the integrals. Results for the two terms in (16.97) are
and
(\(\eta _+(t)\) is the Heaviside unit step function and i, j=1, 2). In the calculation of the expressions given by (16.98), (16.99) and (16.100), we have also used
and
which we found during the calculations [21].
Hence, (16.98) along with (16.99) and (16.100) provide the complete solution for the integral I, which is the time representation of the second term of the full Green’s function \(\mathcal {G}(x_1,x_2; t)_{K}\) given in (16.69).
Rights and permissions
Copyright information
© 2022 The Author(s), under exclusive license to Springer Nature Switzerland AG
About this chapter
Cite this chapter
Horing, N.J.M., Ayyubi, R.A.W., Sabeeh, K., Bahrami, S. (2022). Quantum Dynamics in a 1D Dot/Antidot Lattice: Landau Minibands and Graphene Wave Packet Motion in a Magnetic Field. In: Ünlü, H., Horing, N.J.M. (eds) Progress in Nanoscale and Low-Dimensional Materials and Devices. Topics in Applied Physics, vol 144. Springer, Cham. https://doi.org/10.1007/978-3-030-93460-6_16
Download citation
DOI: https://doi.org/10.1007/978-3-030-93460-6_16
Published:
Publisher Name: Springer, Cham
Print ISBN: 978-3-030-93459-0
Online ISBN: 978-3-030-93460-6
eBook Packages: Physics and AstronomyPhysics and Astronomy (R0)