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Sulfur-Containing Polymer Cathode Materials for Li–S Batteries

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Advances in Rechargeable Lithium–Sulfur Batteries

Part of the book series: Modern Aspects of Electrochemistry ((MAOE,volume 59))

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Abstract

Due to high energy density and low cost of sulfur, lithium-sulfur batteries are of great promise to substitute for lithium-ion batteries in a variety of applications, ranging from electric vehicles to portable electronics. Unfortunately, while providing many advantages, sulfur also has several fatal problems, including poor electronic conductivity, huge volume variation upon charge/discharge, and shuttle effect of polysulfides. Utilizing sulfur-containing polymers rather than elemental sulfur as cathode materials for lithium-sulfur batteries received tremendous attention in recent years. Sulfur species are confined in sulfur-containing polymers via covalent bonds, which can greatly alleviate the shuttle effect and thus render lithium-sulfur batteries improved discharge capacity, enhanced rate capability, and high cycling stability. In this chapter, a comprehensive review on the recent development of sulfur-containing polymer cathodes is provided. Different electrochemical behaviors and different molecular structures of sulfur-containing polymer cathode materials are systematically summarized. Furthermore, the optimization strategies for sulfur-containing polymer cathodes are discussed in detail. Finally, the remaining problems and future prospects for sulfur-containing polymer cathodes are outlined.

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Acknowledgements

Prof. G. Wang would like to acknowledge the support by the Australian Research Council (ARC) Discovery Projects (DP200101249 and DP210101389).

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Authors and Affiliations

  1. School of Mathematical and Physical Sciences, Research Centre for Clean Energy Technology, University of Technology Sydney, Ultimo, Australia

    Yizhou Wang, Dong Zhou & Guoxiu Wang

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  1. Yizhou Wang
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  2. Dong Zhou
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Correspondence to Guoxiu Wang .

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Editors and Affiliations

  1. Materials Science & Engineering, University of Texas at Austin, Austin, TX, USA

    Arumugam Manthiram

  2. College of Chemistry, Zhengzhou University, Zhengzhou, China

    Yongzhu Fu

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Wang, Y., Zhou, D., Wang, G. (2022). Sulfur-Containing Polymer Cathode Materials for Li–S Batteries. In: Manthiram, A., Fu, Y. (eds) Advances in Rechargeable Lithium–Sulfur Batteries. Modern Aspects of Electrochemistry, vol 59. Springer, Cham. https://doi.org/10.1007/978-3-030-90899-7_8

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