Abstract
Nanostructured N-doped TiO2 photocatalyst has been prepared via a new approach from Ti-based MOF[NH2-MIL-125(Ti)] precursor. The success of N do** enhances light absorption and narrows the bandgap. Moreover, the as-prepared nanostructure is constructed with tiny nanoparticles and resembles a pie-like morphology inherited from the MOF, which accelerates electron transfer. Hence, as a photocatalyst for the degradation of methylene blue(MB) under visible light irradiation, the N-doped TiO2(N-TiO2) nanostructure shows higher photocatalytic activity with a reaction rate constant of 0.018 min−1 than that of the TiO2-P25 and TiO2 under the visible light.
Similar content being viewed by others
References
Oar-Arteta L., Wezendonk T., Sun X. H., Kapteijn F., Gascon J., Mater. Chem. Front., 2017, 1(9), 1709
Li X., Yao J. H., Qi J. Y., Chem. Res. Chinese Universities, 2007, 23(2), 273
Wang J. L., Yi Y. J., Li M. J., Chang Y., Zha F., Chem. Res. Chinese Universities, 2019, 35(2), 319
Chen, J. F., Chen X. Y., Zhang X., Yuan Y., Bi R. Y., You F. F., Wang Z. M., Yu R. B., Chem. Res. Chinese Universities, 2020, 36(1), 120
Reutergådh L. B., Iangphasuk M., Chemosphere, 1997, 35(3), 585
Herrmann J. M., Disdier J., Pichat P., Malatoet S., Blancoal J., Appl. Catal, B, 1998, 17(1/2), 15
Zhang J. L., Wu Y. M., **ng M. Y., Khan Leghari A. K., Sajjad S., Energy Environ. Sci., 2010, 3, 715
Ren H., Sun J. J., Yu R. B., Yang M., Gu L., Liu P. R., Zhao H. J., Kisailus D., Wang D., Chem. Sci., 2016, 7, 793
Wang H., **ao L. G., Wang C., Lin B., Lyu S., Chu X. F., Chi Y. D., Yang X. T., Wang X. Y., Chem. Res. Chinese Universities, 2019, 35(4), 667
Chen D. W., Shi J. E., Yan J. C., Wang Y. H., Yan F. C., Shang S. X., Xue J., Chem. Res. Chinese Universities, 2008, 24(2), 362
Li X. Z., Liu H. L., Yue P. T., Sun Y. P., Environ. Sci. Technol., 2000, 34(20), 4401
Ren W. J., Ai Z. H., Jia F. L., Zhang L. Z., Fan X. X., Zou Z. G., Appl. Catal., B, 2007, 69(3/4), 138
Wei Y. Z., Wan J. W., Yang N. L., Ma Y. W., Wang S. C., Wang J. Y., Yu R. B., Lin G., Wang L. H., Wang L. Z., Huang W., Wang D., National Science Review, 2020, DOI: https://doi.org/10.1093/nsr/nwaa059
** Q., Li Z. W., Lin K. F., Wang S., Xu R. G., Wang D., RSC Adv., 2014, 4(84), 44692
Yang Y., ** Q., Mao D., Qi J., Wei Y. Z., Yu R. B., Li A., Li S. Z., Zhao H. J., Ma Y. W., Wang L. H., Hu W. P., Wang D., Adv. Mater., 2017, 29(4), 1604795
Zhang H. J., Chen G. H., Bahnemann D. W., J. Mater. Chem., 2009, 19(29), 5089
de Tacconi N. R., Chenthamarakshan C. R., Rajeshwar K., Pauporté T., Lincot D., Electrochem. Commun., 2003, 5(3), 220
Choi Y., Umebayashi T., Yoshikawa M., J. Mater. Sci., 2004, 39(5), 1837
Diwald O., Thompson T. L., Zubkov T., Walck S. D., Yates J. T., J. Phys. Chem. B, 2004, 108(19), 6004
Yu J. C., Yu J., Ho W., Jiang Z. T., Zhang L. Z., Chem. Mater., 2002, 14(9), 3808
Ohno T., Mitsui T., Matsumura M., Chem. Lett., 2003, 32(4), 364
Asahi R., Morikawa T., Ohwaki T., Aoki K, Taga Y., Science, 2001, 293, 269
Ansari S. A., Khan M. M., Ansari M. O., Cho M. H., New J. Chem., 2016, 40(4), 3000
Solakidou M., Giannakas A., Georgiou Y., Boukos N., Louloudi M., Deligiannakis Y., Appl. Catal., B, 2019, 254, 194
Kitano M., Funatsu K., Matsuoka M., Ueshima M., Anpo M., J. Phys. Chem. B, 2006, 110, 25266
Maeda M., Watanabe T., Electrochem J., Soc., 2006, 153, C186
Wang Z. M., Yang N. L., Wang D., Chem. Sci., 2020, DOI: https://doi.org/10.1039/D0SC01284J
Yuan Y., Chen X. Y., Zhang X., Wang Z. M., Yu R. B., Chen, Inorg. Chem. Front., 2020, DOI: https://doi.org/10.1039/d0qi00023j
Wang Z. M., Gu L., Song L., Wang H., Yu R. B., Mater. Chem. Front., 2018, 2, 1024
Shen Y., Bao L. W., Sun F. Z., Hu T. L., Mater. Chem. Front., 2019, 3(11), 2363
Dan-Hardi M., Serre C., Frot T., Rozes L., Maurin G., Sanchez C., Férey G., J. Am. Chem. Soc., 2009, 131(31), 10857
Kim S. N., Kim J., Kim H. Y., Cho H. Y., Ahn W. S., Catal. Today, 2013, 204, 85
Ranjit K. T., Willner I., Bossmann S. H., Braun A. M., J. Catal., 2001, 204(2), 305
Parida K. M., Sahu N., J. Mol. Catal. A: Chem., 2008, 287, 151
**e Y. B., Yuan C. W., Li X. Z., Colloids Surf., A, 2005, 252(1), 87
D’Arienzo M., Scotti R., Wahba L., Battocchio C., Bemporad E., Nale A., Morazzoni F., Appl. Catal., B, 2009, 93, 149
Zhang H. R., Tan K. Q., Zheng H. W., Gu Y. Z., Zhang W. F., Mater. Chem. Phys., 2011, 125(1/2), 156
Asahi R., Morikawa T., Ohwaki T., Aoki K., Taga Y., Science, 2001, 293(5528), 269
Yeung K. L., Yau S. T., Maira A. J., Coronado J. M., Soria J., Yue P. L., J. Catal., 2003, 219(1), 107
Berger H., Tang H., Lévy F., J. Cryst. Growth, 1993, 130(1/2), 108
Porto S. P. S., Fleury P. A., Damen T. C., Phys. Rev., 1967, 154(2), 522
Bersani D., Lottici P. P., Ding X. Z., Appl. Phys. Lett., 1998, 72(1), 73
Liu S. X., Chen X. Y., Li X. H., Chin. J. Inorg. Chem., 2008, 24(2), 253
Luo W. J., Yang Z. S., Li Z. S., Zhang J. Y., Liu J. G., Zhao Z. Y., Wang Z. Q., Yan S. C., Yu T., Zou Z. G., Energy Environ. Sci., 2011, 4(10), 4046
Yin S., Yamaki H., Zhang Q., Komatsu M., Wang J., Tang Q., Saito F., Sato T., Solid State Ionics, 2004, 172(1—4), 205
Liu H. J., Liu G. G., **e G. H., Zhang M. L., Hou Z. H., He Z. W., Appl. Surf. Sci., 2011, 257(8), 3728
Author information
Authors and Affiliations
Corresponding authors
Additional information
Supported by the National Natural Science Foundation of China(Nos.21671016, 51872024, 51932001), the National Key R&D Program of China(No.2018YFA0703503) and the China Postdoctoral Science Foundation(No.2019M650849).
Electronic supplementary material
Rights and permissions
About this article
Cite this article
He, Y., Zhang, X., Wei, Y. et al. Ti-MOF Derived N-Doped TiO2 Nanostructure as Visible-light-driven Photocatalyst. Chem. Res. Chin. Univ. 36, 447–452 (2020). https://doi.org/10.1007/s40242-020-0106-2
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s40242-020-0106-2