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Ti-MOF Derived N-Doped TiO2 Nanostructure as Visible-light-driven Photocatalyst

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Abstract

Nanostructured N-doped TiO2 photocatalyst has been prepared via a new approach from Ti-based MOF[NH2-MIL-125(Ti)] precursor. The success of N do** enhances light absorption and narrows the bandgap. Moreover, the as-prepared nanostructure is constructed with tiny nanoparticles and resembles a pie-like morphology inherited from the MOF, which accelerates electron transfer. Hence, as a photocatalyst for the degradation of methylene blue(MB) under visible light irradiation, the N-doped TiO2(N-TiO2) nanostructure shows higher photocatalytic activity with a reaction rate constant of 0.018 min−1 than that of the TiO2-P25 and TiO2 under the visible light.

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Correspondence to Zumin Wang or Ranbo Yu.

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Supported by the National Natural Science Foundation of China(Nos.21671016, 51872024, 51932001), the National Key R&D Program of China(No.2018YFA0703503) and the China Postdoctoral Science Foundation(No.2019M650849).

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He, Y., Zhang, X., Wei, Y. et al. Ti-MOF Derived N-Doped TiO2 Nanostructure as Visible-light-driven Photocatalyst. Chem. Res. Chin. Univ. 36, 447–452 (2020). https://doi.org/10.1007/s40242-020-0106-2

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  • DOI: https://doi.org/10.1007/s40242-020-0106-2

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