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Emerging low-density polyethylene/paraffin wax/aluminum composite as a form-stable phase change thermal interface material

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Abstract

Thermal interface materials (TIMs) play a vital role in the thermal management of electronic devices and can significantly reduce thermal contact resistance (TCR). The TCR between the solid-liquid contact surface is much smaller than that of the solid-solid contact surface, but conventional solid-liquid phase change materials are likely to cause serious leakage. Therefore, this work has prepared a new form-stable phase change thermal interface material. Through the melt blending of paraffin wax (PW) and low-density polyethylene (LDPE), the stability is improved and it has an excellent coating effect on PW. The addition of aluminum (Al) powder improves the low thermal conductivity of PW/LDPE, and the addition of 15wt% Al powder improves the thermal conductivity of the internal structure of the matrix by 67%. In addition, the influence of the addition of Al powder on the internal structure, thermal properties, and phase change behavior of the PW/LDPE matrix was systematically studied. The results confirmed that the addition of Al powder improved the thermal conductivity of the material without a significant impact on other properties, and the thermal conductivity increased with the increase of Al addition. Therefore, morphologically stable PW/LDPE/Al is an important development direction for TIMs.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China, China (No. 51874047), the Key Science and Technology Project of Changsha City, China (No. kq2102005), the Special Fund for the Construction of Innovative Province in Hunan Province, China (No. 2020RC3038), and the Changsha City Fund for Distinguished and Innovative Young Scholars, China (No. kq1802007).

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Authors and Affiliations

  1. School of Energy and Power Engineering, Changsha University of Science and Technology, Changsha, 410114, China

    Chuanchang Li & Weixuan Wang

  2. Shenzhen Institute of Advanced Electronic Materials, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen, 518055, China

    **aoliang Zeng & Rong Sun

  3. Hunan **angtou Light Material Technology Co., Ltd., Changsha, 410012, China

    Chunxuan Liu

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  1. Chuanchang Li
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Correspondence to Chuanchang Li.

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Li, C., Wang, W., Zeng, X. et al. Emerging low-density polyethylene/paraffin wax/aluminum composite as a form-stable phase change thermal interface material. Int J Miner Metall Mater 30, 772–781 (2023). https://doi.org/10.1007/s12613-022-2565-6

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