Abstract
The advantages of efficient and flexible digital printing are tempered by the serious environmental impact of many synthetic dyes and chemicals. In response to this problem, we prepared cyan, magenta, yellow, and black (CMYK) inks using biodegradable natural dyes for inkjet printing, including gardenia blue, amaranth, gardenia yellow, logwood, and lac. We monitored the prepared inks for 60 days for storage stability evaluation. In addition, we evaluated the printing quality by measuring color strength (K/S), ink penetration, printing sharpness, and color fastness in cotton and silk fabrics. The unique color of each prepared ink was printed well, with good storage stability and excellent printing sharpness. The printing sharpness of cotton fabrics was better than that of silk fabrics. On the other hand, the penetration factor value of silk printing was significantly greater than that of cotton printing. The rubbing fastness and washing fastness were very good for both cotton and silk fabrics. The light fastness of magenta and black ink on silk fabrics was excellent at rating 4/5, but that of cyan ink on cotton and silk was low at rating 2. In addition to CMYK's unique colors, various colors and line images such as flowers, cherries, and leaves could be printed clearly and delicately on the fabric. This study provides a useful model in the textile printing ink field to assess natural dye inks, which are rarely produced. Fabrics using biodegradable natural dyes inks are less destructive to the environment than synthetic dye inks. Another benefit is that the fabrics are harmless to humans and unlikely cause allergies in people with sensitive skin.
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig1_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig2_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig3_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig4_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig5_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig6_HTML.png)
![](http://media.springernature.com/m312/springer-static/image/art%3A10.1007%2Fs12221-023-00162-3/MediaObjects/12221_2023_162_Fig7_HTML.png)
Similar content being viewed by others
References
B. Tawiah, E.K. Howard, B.K. Asinyo, Int. J. Manag. Inf. Technol. Eng. 4(5), 61 (2016)
S. Magdassi, The Chemistry of Ink Jet Inks (Singapore World Scientific Publishing Co Pte Ltd, Singapore, 2010), pp.3–9
H. Ujiie, Digital printing of textiles, 4th edn. (Woodhead Publishing, Cambridge, 2006), pp.293–301
S. Faisal, A. Tronci, Fibers Polym. 19, 1435 (2018)
S.K. Malik, S. Kadian, S. Kumar, Indian J. Fibre Text. Res. 30(1), 99 (2005)
H. Ujiie, Digital Printing of Textiles, 3rd edn. (Woodhead Publishing, Cambridge, 2006), pp.212–214
Y. Song, K. Fang, M.N. Bukhari, Y. Ren, K. Zhang, Z. Tang, A.C.S. Appl, Mater. Interfaces 12, 45281 (2020)
G. Savvidis, E. Karanikas, N. Nikolaidis, I. Eleftheriadis, E. Tsatsaroni, Color. Technol. 130, 200 (2014)
J.Y. Park, Y. Hirata, K. Hamada, Color. Technol. 128, 184 (2012)
G.L. Gungor, A. Kara, D. Gardini, M. Blosi, M. Dondi, C. Zanelli, Dyes Pigm. 127, 148 (2016)
X. Hou, G. Chen, T. **ng, Z. Wei, Eng. Fibers Fabr. 14, 1 (2019). https://doi.org/10.1177/1558925019849242
Z. Tang, K. Fang, M.N. Bukhari, Y. Song, K. Zhang, Langmuir 36, 9481 (2020)
Z. Stempien, M. Khalid, M. Kozicki, M. Kozanecki, H. Varela, P. Filipczak, R. Pawlak, E. Korzeniewska, E. Sasiadek, Synth. Met. 256, 116144 (2019)
M. Li, L. Zhang, D. Wang, C. Agbo, S. Fu, Color. Technol. 133, 476 (2017)
S. Leelajariyakul, H. Noguchi, S. Kiatkamjornwong, Prog. Org. Coat. 62, 145 (2008)
S. Daplyn, L. Lin, Pigm. Resin Technol. 32, 307 (2003)
M.M. Marie, Y.H. El-Hamaky, D. Maamoun, D.F. Ibrahim, S.M. Abbas, IJIAS 4, 239 (2013)
M.N. Karim, M. Rigout, S.G. Yeates, C. Carr, Dyes Pigm. 103, 168 (2014)
H. Shahariar, I. Kim, H. Soewardiman, J.S. Jur, A.C.S. Appl, Mater. Interfaces 11, 6208 (2019)
J. Kastner, T. Faury, H.M. Außerhuber, T. Obermüller, H. Leichtfried, M.J. Haslinger, E. Liftinger, J. Innerlohinger, I. Gnatiuk, D. Holzinger, T. Lederer, Microelectron. Eng. 176, 84 (2017)
S. Merilampi, T. Laine-Ma, P. Ruuskanen, Microelectron. Reliab. 49, 782 (2009)
X. Nie, H. Wang, J. Zou, Appl. Surf. Sci. 261, 554 (2012)
A. Karolia, H. Buch, Indian J. Tradit. Knowl. 7(1), 93 (2008)
S. Bains, M. Sethi, Man-made Text. India 47(11), 380 (2019)
O.A. Hakeim, A. Abou-Okeil, L.A.W. Abdou, A. Waly, J. Appl. Polym. Sci. 97, 559 (2005)
A.A. Hebeish, A.A. Ragheb, S.H. Nassar, E.E. Allam, J.I. Abd El Thalouth, J. Appl. Polym. Sci. 102, 338 (2006)
G. Savvidis, V. Karanikas, M. Zarkogianni, I. Eleftheriadis, N. Nikolaidis, E. Tsatsaroni, J. Nat. Fibers 14, 326 (2016)
S. Babel, R. Gupta, J. Text. Sci. Eng. 6, 1000230 (2016)
R. Mongkholrattanasit, C. Klaichoi, N. Sasithorn, W. Changmuang, K. Manarungwit, K. Maha-In, P. Ruenma, N. Boonkerd, N. Sangaphat, M. Pangsai, Vlakna a textil 3, 51 (2018)
M. Kavyashree, in Chemistry and technology of natural and synthetic dyes and pigments, 8th edn., ed. by A.K. Samanta, N. Awwad, H.M. Algarni (IntechOpen publisher, London, 2020), pp.195–204
O.A. Hakeim, S.H. Nassar, K. Haggag, Indian J. Fibre Text. Res. 28, 216 (2003)
S.M. Vega Gutierrez, Y. He, Y. Cao, D. Stone, Z. Walsh, R. Malhotra, H.L. Chen, C.H. Chang, S.C. Robinson, Coatings 9(4), 266 (2019)
L. Wang, Q. Zhu, H. Yu, G. **e, Z. Yu, Ind. Crops. Prod. 187, 115490 (2022)
A.M. Thakker, D. Sun, D. Bucknall, Environ. Sci. Pollut. Res. 29, 68357 (2022)
J.C. Briggs, A.H. Klein, M.K. Tse, Applications of ISO–13660, a new international standard for objective print quality evaluation/ISJ (Hardcopy, Japan, 1999)
C.W. Kan, C.W.M. Yuen, W.Y. Tsoi, Cellulose 18, 827 (2011)
H. Yang, K. Fang, X. Liu, Y. Cai, F. An, Polymers 10, 1219 (2018)
X. Wang, Y. Yin, C. Wang, Colloids Surf. A: Physicochem. Eng. Asp. 361, 51 (2010)
H. Cao, L. Ai, Z. Yang, Y. Zhu, Polymers 11, 1504 (2019)
S. Faisal, M. Ali, S.H. Siddique, L. Lin, Pigm. Resin Technol. 50, 285 (2021)
Y.F. Liu, M.H. Tsai, Y.F. Pai, W.S. Hwang, Appl. Phys. A 111, 509 (2013)
C.W. Kan, C.W.M. Yuen, Res. J. Text. Appar. 16(2), 1 (2012)
C. Cie, Ink Jet Textile Printing, 8th edn. (Woodhead Publishing, Cambridge, 2015)
A.W. Kaimouz, R.H. Wardman, R.M. Christie, Color. Technol. 126, 342 (2010)
H. Ujiie, Digital Printing of Textiles, 3rd edn. (Woodhead Publishing, Cambridge, 2006), pp.260–274
Author information
Authors and Affiliations
Corresponding author
Ethics declarations
Conflict of Interest
This manuscript has not been published or presented elsewhere in part or entirely and is not under consideration by any other journal. Co-authors provided informed consent for all study. We have read and understood your journal’s policies. We believe that neither the manuscript nor the study violates any of these. There are no conflicts of interest to declare.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Yeo, Y., Shin, Y. Inkjet Printing of Textiles Using Biodegradable Natural Dyes. Fibers Polym 24, 1695–1705 (2023). https://doi.org/10.1007/s12221-023-00162-3
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s12221-023-00162-3