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Progress and perspective on rechargeable magnesium-ion batteries

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Abstract

Current electrochemical energy storage technology has evolved a variety of rechargeable battery systems. Recently, the resource shortage of raw materials in commercially available lithium-ion batteries has attracted widespread attention. The requirements to meet resourcefulness, sustainability, safety, and high energy density have motivated the development of rechargeable magnesium-ion batteries (RMBs). Although RMBs have made significant progress so far, there are still many obstacles to practical orientation. We systematically summarize the significant progress and the latest research on RMBs, including Mg2+-conducting electrolytes, Mg2+-storage cathodes, and Mg-based anodes. In this review, we mainly introduce the properties and features of various Mg2+-conductive electrolytes, the mainstream cathode materials, and their respective Mg2+-storage mechanisms, as well as the Mg metal (or alloy) anodes and the corresponding modification strategies. Finally, the future directions in various key components for RMBs are highlighted.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (22179135, 22109168, 52072195, and 21975271), the Strategic Priority Research Program of the Chinese Academy of Sciences (XDA22010603, XDA22010600), Taishan Scholars Program for Young Expert of Shandong Province (tsqn202103145), Shandong Energy Institute (SEI I202108 and SEI I202127) and the China Postdoctoral Science Foundation (BX20200344, 2020M682251).

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  1. School of Materials Science and Engineering, Ocean University of China, Qingdao, 266100, China

    Guixin Wang, Zhechen Wang & Mingliang Sun

  2. Qingdao Industrial Energy Storage Research Institute, Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Qingdao, 266101, China

    Guixin Wang, Hucheng Shi, Aobing Du & Guanglei Cui

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Wang, G., Wang, Z., Shi, H. et al. Progress and perspective on rechargeable magnesium-ion batteries. Sci. China Chem. 67, 214–246 (2024). https://doi.org/10.1007/s11426-022-1454-0

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