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Effect of Ni do** on the microstructure and electrical properties of Ba–Co–O NTC ceramics

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Abstract

A novel perovskite BaNixCo1‒xO3‒δ (0 ≤ x ≤ 0.1) Negative Temperature Coefficient thermal ceramic material has been successfully synthesized using a solid-phase method. The XRD analysis revealed that the BaNixCo1‒xO3‒δ ceramics possess a hexagonal perovskite structure. Moderate do** with Ni ions facilitates high density in this perovskite ceramic material. The grain size exhibits a pattern of initially increasing and then decreasing with the addition of Ni2+ do**. The electrical resistivity of the perovskite ceramic material decreases and then increases with Ni2+ do**. The electrical conductivity mechanism of perovskite ceramic materials is consistent with the Mott VRH model in the temperature range below 105 K and the thermally activated conduction model in the 105–300 K temperature range. The resistivity, activation energy, and material constant B values of the ceramic material at 125 K range from 50.86–68.09 Ω·cm, 50.45–60.07 meV, and 652.79–687.02 K. A ceramic material with low B value and low resistance was developed for thermal applications, with a measurement temperature range of 10–300 K. The material shows promise for application in the specialized environmental monitoring industry.

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Data availability

The data that support the findings of this study are available from the corresponding author upon reasonable request.

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Funding

This work was supported by the Western Light Program of the Chinese Academy of Sciences (Grant numbers: 2021-XBQNXZ-019) and the Science and Technology Development Project of Two zones **njiang (Grant No. 2022LQ03006).

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Authors and Affiliations

  1. Key Laboratory of Functional Materials and Devices Under Special Environments of CAS, **njiang Key Laboratory of Electronic Information Materials and Devices, **njiang Technical Institute of Physics & Chemistry of CAS, Urumqi, 830011, China

    Hao Wang, Shuangji Feng, Yaohua Li, Yuling Tuo, Pengjun Zhao, Yi Liu, **a Huang & Aimin Chang

  2. School of Physics Science and Technology, **njiang University, Ürümqi, 830046, China

    Hao Wang & Shuangji Feng

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  1. Hao Wang
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  2. Shuangji Feng
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  3. Yaohua Li
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Contributions

WH: Conceptualization (equal); Data curation (lead); Formal analysis (lead); Methodology analysis (lead); Investigation(equal); Visualization (equal); Writing-original draft (lead). SF: Data curation (supporting); Methodology (supporting). YL: Conceptualization (supporting); Formal analysis (supporting); Investigation (supporting). YT: Formal analysis (supporting); Methodology (supporting). PZ: Formal analysis (supporting); Investigation (supporting); Methodology (supporting). YL: Formal analysis (equal); Methodology (supporting); Software (supporting); Visualization (lead). XH: Conceptualization (lead); Data curation (supporting); Formal analysis (equal); Funding acquisition (lead); Investigation (equal); Supervision (lead); Writing-review and editing(equal). AC: Project administration (equal); Resources (supporting); Validation (equal).

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Correspondence to **a Huang or Aimin Chang.

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Wang, H., Feng, S., Li, Y. et al. Effect of Ni do** on the microstructure and electrical properties of Ba–Co–O NTC ceramics. J Mater Sci: Mater Electron 35, 1294 (2024). https://doi.org/10.1007/s10854-024-13044-y

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