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Single-source-precursor synthesized SiCN/MWCNT nanocomposites with improved microwave absorbing performance

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Abstract

To improve the microwave absorbing performance, SiCN/MWCNT nanocomposites with different carboxylic functionalized multi-walled carbon nanotubes (MWCNT-COOH) contents (0 wt%, 2 wt%, 4 wt% and 8 wt%) were synthesized by single-source-precursor poly(methylvinyl)silazane (HTT1800) and polymer-derived ceramics method. The microwave absorbing performance of SiCN/MWCNT nanocomposites were investigated in the frequency range of 8.2–12.4 GHz with the thickness varied from 3.0 to 5.0 mm. The results showed that the minimum reflection loss (RLmin) of the sample of 10 wt% SiCN/MWCNT-8 mixed with paraffin wax reached − 30.34 dB with the thickness of 4.5 mm in the frequency of 11.45 GHz. The reason was that the introduction of MWCNT-COOH increased the interfacial polarization loss and the conduction loss of nanocomposites, improving microwave absorbing performance. The findings demonstrated that the synthesized SiCN/MWCNT nanocomposites possessed promising prospects as microwave absorbing materials.

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The datasets generated during and/or analyzed during the current study are available from the corresponding author on reasonable request.

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Funding

This work was supported by the General Project (Youth) of Shaanxi Provincial Natural Science Basic Research Program (Grant No. 2023-JC-QN-0523), Scientific Research Plan Projects of Shaanxi Education Department (Grant No. 22JK0426), **’an Postdoctoral Innovation Base (Grant No. 2021-1), School-level Scientific Research Fund of **’an Aeronautical University (Grant No. 2021KY0201).

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Authors and Affiliations

  1. School of Materials Engineering, **’an Aeronautical University, **’an, 710077, China

    Beibei Wang

  2. Shaanxi Province Key Laboratory of Fiber Reinforced Light Composite Materials, Northwestern Polytechnical University, **’an, 710072, China

    Beibei Wang, Yue Liu & Qiangang Fu

  3. Department of Materials and Earth Sciences, Technical University of Darmstadt, 64287, Darmstadt, Germany

    Beibei Wang, **ngmin Liu & Ralf Riedel

Authors
  1. Beibei Wang
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  2. **ngmin Liu
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  3. Yue Liu
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  4. Qiangang Fu
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  5. Ralf Riedel
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Contributions

The team members are contributed based on the following roles: BW: Conceptualization, Methodology, Investigation and Writing-Original draft preparation. XL: Conceptualization, Methodology. YL: Project administration, Conceptualization, Methodology, Resources, Visualization, Supervision, Writing-Reviewing and Editing. QF: Supervision. RR: Supervision, Writing-Reviewing and Editing.

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Correspondence to Beibei Wang.

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Wang, B., Liu, X., Liu, Y. et al. Single-source-precursor synthesized SiCN/MWCNT nanocomposites with improved microwave absorbing performance. J Mater Sci: Mater Electron 35, 125 (2024). https://doi.org/10.1007/s10854-024-11941-w

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