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Dynamic shock wave-induced switchable order to disorder states of single crystal of sulfamic acid: a combined study of X-ray and Raman spectroscopy

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Abstract

Experimentation under dynamic shocked conditions has attained the status of one of the appealing classes of methods for identifying the functional materials whose degree of long-range order is significantly altered. In the present work, we have systematically investigated the dynamic impact of shock waves on the technologically important single crystal of sulfamic acid at various numbers of shocks exposed and the results have been analyzed by X-ray diffraction and Raman spectroscopic profiles. Based on the obtained results, the shocked phase profile with respect to the number of shock pulses is of the sequential order (Pbca)–disorder–order (Pbca)–disorder–order (Pbca) for the 0, 1, 2, 3 and 4 shocks, respectively. The observed switchable phase transitions of the titled crystal after shocked conditions might be due to the rotational order–disorder transformation that is followed by the molecular symmetry changes of NH3 and SO3 trigonal units for which the possible macroscopic mechanism is provided. The observed switchable phase transitions occurring between order and disorder states may be an interesting asset for molecular electronic devices such as the molecular switches.

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Acknowledgements

The authors thank Sacred Heart College for Don Bosco Research Grant (SHC/DB Grant/2021/01) and NSF of China (42072055). The project was supported by Researchers Supporting Project number (RSP2023R142), King Saud University, Riyadh, Saudi Arabia.

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Authors and Affiliations

  1. Key Laboratory of High-Temperature and High-Pressure Study of the Earth’s Interior, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang, 550081, Guizhou, China

    A. Sivakumar & Lidong Dai

  2. Department of Physics, Kings Engineering College, Sriperumbudur, Chennai, Tamilnadu, 602 117, India

    S. Sahaya Jude Dhas

  3. Department of Physics, JCT College of Engineering and Technology, Coimbatore, Tamilnadu, 641 105, India

    J. Thirupathy

  4. Department of Materials Science, School of Technology, Central University of Tamil Nadu, Thiruvarur, Tamilnadu, 610 005, India

    K. Sethuraman

  5. Department of Chemistry, College of Science, King Saud University, P.O. Box 2455, Riyadh, 11451, Saudi Arabia

    Raju Suresh Kumar & Abdulrahman I. Almansour

  6. CSIR-National Physical Laboratory, Dr. K.S. Krishnan Road, New Delhi, 110 012, India

    N. Vijayan

  7. Shock Wave Research Laboratory, Department of Physics, Abdul Kalam Research Center, Sacred Heart College, Tirupattur, Vellore, Tamil Nadu, 635 601, India

    S. A. Martin Britto Dhas

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  1. A. Sivakumar
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Correspondence to A. Sivakumar, Lidong Dai or S. A. Martin Britto Dhas.

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Sivakumar, A., Dhas, S.S.J., Dai, L. et al. Dynamic shock wave-induced switchable order to disorder states of single crystal of sulfamic acid: a combined study of X-ray and Raman spectroscopy. J Mater Sci 58, 8415–8425 (2023). https://doi.org/10.1007/s10853-023-08532-1

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