Abstract
We provide guidelines to femtosecond laser users to select ad hoc laser parameters, namely the fluence and pulse duration, in the context of the development of ablation processes at the surface of dielectrics using single femtosecond pulses. Our results and discussion are based on a comprehensive experimental and theoretical analysis of the energy deposition process at the surface of fused silica samples and of their postmortem ablation characteristics, in the range of intensities from 1013 to 1015 W/cm2. We show experimentally and numerically that self-induced plasma transient properties at the pulse timescale dramatically determine the efficiency of energy deposition and affect the resulting ablation morphology. In practice, we determine that the precise measurement of two characteristic fluence values, namely the laser-induced ablation threshold F th,LIAT and the fluence F opt for maximum ablation efficiency, are only required to qualify the outcomes of laser ablation at the surface of a dielectric in an extended range of applied fluence.
Similar content being viewed by others
References
R. Gattass, E. Mazur, Nat. Phot. 2, 219 (2008)
S. Juodkazis, V. Mizeikis, H. Mizawa, J. Appl. Phys. 106, 051101 (2009)
S.H. Chung, E. Mazur, J. Biophoton. 2(10), 557 (2009)
F. Dausinger, F. Lichtner, H. Lubatschowski, Femtosecond Technology for Technical and Medical Applications (Springer, Berlin, 2004)
E. Stratakis, A. Ranella, M. Farsari, C. Fotakis, Prog. Quantum Electron. 33, 127 (2009)
C. Rullière (ed.), Femtosecond Laser Pulses: Principles and experiments, 2nd edn. (Springer, Berlin, 2003)
J.-C. Diels, W. Rudolph, Ultrashort Laser Pulse Phenomenon: Fundamentals, Techniques and Applications on a Femtosecond Time Scale (Academic, Boston, 1996)
E. Gamaly, Femtosecond Laser-Matter Interactions (Pan Stanford Publishing, Singapore, 2011)
M.D. Perry, B.C. Stuart, P.S. Banks, M.D. Feit, V. Yanovsky, A.M. Rubenchik, J. Appl. Phys. 85(9), 6803 (1999)
K. Sugioka, Y. Cheng (eds.), Ultrafast Laser Processing: From Micro- to Nanoscale (Pan Stanford Publishing, Singapore, 2013)
W. Sibbett, A.A. Lagatsky, C.T.A. Brown, Opt. Exp. 20(7), 6989 (2012)
P. Martin, S. Guizard, Ph Daguzan, G. Petite, P. D’Oliveira, P. Meynadier, M. Perdrix, Phys. Rev. B 55(9), 5799 (1997)
R. Stoian, A. Rosenfeld, D. Ashkenasi, I.V. Hertel, N.M. Bulgakova, E.E.B. Campbell, Phys. Rev. B 88(9), 097603 (2002)
M. Li, S. Menon, J.P. Nibarger, G.N. Gibson, Phys. Rev. Lett. 82, 2394 (1999)
A.Q. Wu, I.H. Chowdhury, X. Xu, Phys. Rev. B 72, 085128 (2005)
G.M. Petrov, J. Davis, J. Phys. B At. Mol. Opt. Phys. 41, 025601 (2008)
D. Puerto, J. Siegel, W. Gawelda, M. Galvan-Sosa, L. Ehrentraut, J. Bonse, J. Solis, J. Opt. Soc. Am. B 27, 1065 (2010)
B.C. Stuart, M.D. Feit, S. Herman, A.M. Rubenchik, B.W. Shore, M.D. Perry, Phys. Rev. B 53, 1749 (1996)
L.V. Keldysh, Sov. Phys. JETP 20(5), 1307 (1965)
E.G. Gamaly, A.V. Rode, B. Luther-Davies, V.T. Tikhonchuk, Phys. Plasmas 9(3), 949 (2002)
A. Kaiser, B. Rethfeld, M. Vicanek, G. Simon, Phys. Rev. B 61(17), 11437 (2000)
J.R. Peňano, P. Sprangle, B. Hafizi, W. Manheimer, A. Zigler, Phys. Rev. E 72, 036412 (2005)
M.D. Feit, A.M. Komashko, A.M. Rubenchik, Appl. Phys. A 79, 1657 (2004)
N.M. Bulgakova, R. Stoian, A. Rosenfeld, I.V. Hertel, W. Marine, E.E.B. Campbell, Appl. Phys. A 81, 345 (2005)
C. Mézel, A. Bourgeade, L. Hallo, Phys. Plasmas 17, 113504 (2010)
P. Balling, J. Shou, Rep. Prog. Phys. 76, 036502 (2013)
P.P. Rajeev, D. Gertsvolf, P.B. Corkum, D.M. Rayner, Phys. Rev. Lett. 102, 083001 (2009)
T. Jia, Z. Xu, R. Li, D. Feng, X. Li, C. Cheng, H. Sun, N. Xu, H. Wang, J. Appl. Phys. 95(9), 5166 (2004)
A.M. Weiner, Opt. Commun. 284, 3669 (2011)
T. Brixner, N.H. Damrauer, G. Krampert, P. Niklaus, G. Gerber, J. Opt. Soc. Am. B Opt. Phys. 20(5), 878 (2003)
N. Sanner, N. Huot, E. Audouard, C. Larat, J.-P. Huignard, Opt. Laser. Eng. 45, 737 (2007)
N. Sanner, O. Utéza, B. Bussiere, G. Coustillier, A. Leray, T. Itina, M. Sentis, Appl. Phys. A 94, 889 (2009)
F. Korte, S. Adams, A. Egbert, C. Fallnich, A. Ostendorf, Opt. Exp. 7(2), 41 (2000)
Standard ISO 11254-1, Determination of Laser-Damage Threshold of Optical Surfaces. 1. 1-on-1 test (International Organization for Standardization, Geneva, Switzerland, 2000)
B. Chimier, O. Utéza, N. Sanner, M. Sentis, T. Itina, P. Lassonde, F. Légaré, F. Vidal, J.C. Kieffer, Phys. Rev. B 84, 094104 (2011)
O. Utéza, N. Sanner, B. Chimier, A. Brocas, N. Varkentina, M. Sentis, P. Lassonde, F. Légaré, J.C. Kieffer, Appl. Phys. A 105, 131 (2011)
I.H. Chowdhury, A.Q. Wu, X. Xu, A.M. Weiner, Appl. Phys. A 81, 1627 (2005)
S.C. Rae, K. Burnett, Phys. Rev. A 46, 1084 (1992)
D. Grojo, M. Gertsvolf, S. Lei, T. Barillot, D.M. Rayner, P.B. Corkum, Phys. Rev. B 81, 212301 (2010)
L. Jiang, H.L. Tsai, J. Appl. Phys. 104, 093101 (2008)
M. Lenzner, J. Krüger, S. Sartania, Z. Cheng, Ch. Spielmann, G. Mourou, W. Kautek, F. Krausz, Phys. Rev. Lett. 80(18), 4076 (1998)
D. Arnold, E. Cartier, D.J. DiMaria, Phys. Rev. B 49, 10278 (1994)
K. Eidmann, J. Meyer-ter Vehn, T. Schlegel, and S. Hüller, Phys. Rev. E 62, 1202 (2000)
J.D. Huba (ed.), NRL Plasma Formulary (Naval Research Laboratory Publication, Washington, DC, 2005)
A. Belsky, P. Martin, H. Bachau, A.N. Vasil’ev, B.N. Yatsenko, S. Guizard, G. Geoffroy, G. Petite, Europhys. Lett. 67, 301 (2004)
R. Stoian, D. Ashkenasi, A. Rosenfeld, E.E.B. Campbell, Phys. Rev. B 62, 13167 (2000)
Acknowledgments
This research was supported by the French National Agency of Research (ANR) under the contracts “Festic-ANR-06-BLAN-0298-02” and “Nanomorphing-07-BLAN-0301-03” and by the Region Provence–Alpes–Côte d’Azur and Department of Bouches-du-Rhône.
We also thank our colleagues B. Chimier (CELIA, France), T. Itina (LaHC, France) and N. Varkentina (LOMA, France) for stimulating discussions on the results presented in this paper and P. Lassonde, F. Légaré and J.C. Kieffer of INRS-EMT (Québec, Canada) for providing the laser damage setup and their help in performing and interpreting the experiments.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Lebugle, M., Sanner, N., Utéza, O. et al. Guidelines for efficient direct ablation of dielectrics with single femtosecond pulses. Appl. Phys. A 114, 129–142 (2014). https://doi.org/10.1007/s00339-013-8153-x
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s00339-013-8153-x