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Photocatalytic production of H2O2 and its in-situ environmental applications

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Abstract

Hydrogen peroxide (H2O2) is a mild, environmentally friendly, and versatile oxidizer. The current main production process, the anthraquinone method, has high energy consumption and pollution. However, the photocatalytic production of H2O2 is considered to be a green and sustainable process. In this paper, the research progress of photocatalytic production of H2O2 was reviewed. Firstly, the basic principle of photocatalytic production of H2O2 and the three production pathways, namely, oxygen reduction, water oxidation, and dual-channel were introduced. Then, advanced photocatalysts for H2O2 production were introduced with emphasis. From the reactants and products, several new reaction systems and improvement strategies were introduced, including the construction of a spontaneous system without a sacrifice agent, a gas–liquid–solid three-phase system, and inhibition of H2O2 decomposition. The in-situ applications of photocatalytic H2O2 production in the environmental field, including in-situ disinfection and in-situ degradation of pollutants are discussed. Finally, the research progress and future research directions in this field are summarized and prospected.

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Fig. 1
Fig. 2

Copyright 2019 Wiley

Fig. 3
Fig. 4

Copyright 2019 American Chemical Society. c Schematic energy-band diagrams for Au/TiO2, Ag/TiO2, and Au–Ag/TiO2 heterojunction. d Mechanism for photocatalytic production of H2O2 on Au–Ag/TiO2 catalyst [27]. Copyright 2012 American Chemical Society. e Preparation process and surface oxygen reduction mechanism of Pd/APTMS/TiO2 [28]. Copyright 2019 American Chemical Society

Fig. 5

Copyright 2018 Elsevier. c Linear sweep voltammetry with the electrodes of TiO2, TiO2/CoPi, rGO/TiO2, and rGO/TiO2/CoPi [32]. Copyright 2014 Royal Society of Chemistry. d Transient PL spectra of TiO2/Gr samples at 460 nm excitation wavelength. e Uv–vis absorption of TiO2/Gr and TiO2 [34]. Copyright 2022 Wiley. f UV–vis DRS spectra of P25, Ti3C2 MXene, and their composites [36]. Copyright 2021 Elsevier

Fig. 6

Copyright 2021 Royal Society of Chemistry. c S-scheme photocatalytic mechanism in TiO2/In2S3 heterojunction [39]. Copyright 2023 Springer. d S-scheme charge transfer mechanism of TiO2 and PDA [40] Copyright 2022 American Chemical society

Fig. 7

Copyright 2021 Elsevier

Fig. 8

Copyright 2019 American Chemical Society. c different defect structure models of cyano and nitrogen vacancies were introduced successively [54]. Copyright 2022 Royal Society of Chemistry

Fig. 9

Copyright 2021 Wiley

Fig. 10

Copyright 2021 American Chemical Society.

Fig. 11

Copyright 2022 Nature.

Fig. 12

Copyright 2019 Royal Society of Chemistry. b Proposed mechanism for photocatalytic H2O2 production by hydrophobic OPA/Fe-Zr-MOF in a BA/H2O two-phase system [86]. Copyright 2021 American Chemical Society

Fig. 13

Copyright 2022 Wiley. c Free energy diagram of two-electron water oxidization pathway toward H2O2 production on diacetylene linker in CTF-BDDBN [94]. Copyright 2019 Wiley. d Photocatalytic mechanism of H2O2 synthesis in the presence of COF-TfpBpy [96]. Copyright 2022 Wiley

Fig. 14

Copyright 2021 American Chemical Society

Fig. 15

Copyright 2021 Wiley. b O2-TPD spectra and c mechanism of H2O2 photoproduction on Pd/A/BiVO4 [124]. Copyright 2022 American Chemical Society

Fig. 16

Copyright 2021 Elsevier

Fig. 17

Copyright 2022 Elsevier. Copyright 2021 Elsevier. c P-C3N4/O-C3N4 [162] and d mechanism diagram of Fe2(MoO4)3/Ag/Ag3PO4 [163] photocatalytically auto-Fenton reaction. Copyright 2022 Elsevier

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Acknowledgements

This work was financially supported by the National Natural Science Foundation of China (22076046, 22176061), the Science and Technology Commission of Shanghai Municipality (21230712000), the Shanghai Pujiang Program (21PJD016), and the Fundamental Research Funds for the Central Universities (SLB13233301).

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  1. Song Huang and **ngzi Yang have contributed equally to this work.

Authors and Affiliations

  1. Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Feringa Nobel Prize Scientist Joint Research Center, School of Chemistry and Molecular Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, People’s Republic of China

    Song Huang, Lingzhi Wang & **long Zhang

  2. National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery, State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control On Chemical Process, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, People’s Republic of China

    Song Huang, **ngzi Yang, Liang Zhou, Juying Lei & Yongdi Liu

  3. Shanghai Institute of Pollution Control and Ecological Security, Shanghai, 200092, People’s Republic of China

    Liang Zhou & Juying Lei

  4. Shanghai Engineering Research Center for Multi-Media Environmental Catalysis and Resource Utilization, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, People’s Republic of China

    Liang Zhou, Juying Lei & Yongdi Liu

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  1. Song Huang
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Song Huang and **ngzi Yang Wrote original Draft; Liang Zhou and Yongdi Liu reviewed and revised the manuscript; Juying Lei and **long Zhang reviewed and revised the manuscript and provided funding.

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Huang, S., Yang, X., Zhou, L. et al. Photocatalytic production of H2O2 and its in-situ environmental applications. Res Chem Intermed (2024). https://doi.org/10.1007/s11164-024-05301-w

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