Abstract
A series of Ba0.85Ca0.15Zr0.1(Ti1−xNix)0.9O3 (BCZT-xNi) (x = 0, 0.01, 0.02, 0.04) ceramics were prepared by the sol–gel method. The XRD results demonstrate that there is no secondary phase, revealing that Ni completely entered the unit cell to form a solid solution. The microstructures for Ni-doped BCZT ceramics show the average grain size decreases significantly with the increase of Ni content. When x = 0.01, the sample shows relatively high dielectric constant (εr ~ 4473) and good frequency stability, and low dielectric loss at 102 Hz (tan δ ~ 0.004). Influenced by do** Ni, the Curie temperature decreases and the diffusion phase transition increases. The hysteresis loop becomes slimmer and residual polarization is reduced. The sample of x = 0.02 shows an energy density of 0.18 J/cm3 and an energy efficiency of 70.12%. From the present work, cation replacement is an effective way to adjust its ferroelectric, dielectric, and energy storage properties.
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Acknowledgements
This work has been financially supported by the National Natural Science Foundation of China (nos. 51402091, 61901161), the Scientific Research Project in Henan Normal University (no. 20210376), the National University Student Innovation Program (no. 202010476023), and the University Student Innovation Program in Henan Normal University (nos. 20200208, 20200209, 20200212).
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In this article, the author's contributions are as follows, HL: data curation, writing—original draft, visualization. JL: investigation, data curation, writing—review and editing. YS: investigation, resources, writing—original draft. BZ: writing—review and editing, visualization. LL: resources. RL: writing—review and editing. SW: writing—review and editing. XL: writing—review and editing. JS: writing—review and editing. YH: writing—review and editing. XW: conceptualization, writing—review and editing, supervision.
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Li, H.N., Li, J.H., Shi, Y.C. et al. Structure, dielectric, and ferroelectric properties of Ni do** on Ba0.85Ca0.15Zr0.1Ti0.9O3 ceramics. Appl. Phys. A 129, 474 (2023). https://doi.org/10.1007/s00339-023-06758-z
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DOI: https://doi.org/10.1007/s00339-023-06758-z