Abstract
Nuclear reaction analysis (NRA) is a method utilizing an ion beam from an accelerator to determine the hydrogen content in materials. The hydrogen concentration can be quantified absolute and the method can provide depth profiles in the range up to 2–3 μm with a depth resolution in the range of a few nm. Concentrations of 500 at. ppm are easily measurable and with special efforts sensitivities down to 1 ppm have been achieved. The chapter describes the basic principles of the measurements and data analyses and discusses special cases and complications arising with particular samples or when very low concentrations are to be measured.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
Similar content being viewed by others
References
D.A. Leich, T.A. Tombrello, Nucl. Instrum. Methods 108, 67 (1973)
W.A. Lanford, H.P. Trautvetter, J.F. Ziegler, J. Keller, Appl. Phys. Lett. 28, 566 (1976)
W.A. Lanford, Nucl. Instrum. Methods B66, 65 (1992)
H.W. Becker, M. Bahr, M. Berheide, L. Borucki, M. Buschmann, C. Rolfs, G. Roters, S. Schmidt, W.H. Schulte, G.E. Mitchell, J.S. Schweitzer, Z. Phys. A 351, 453 (1995)
Y. Wang, M. Nastasi (eds.), Handbook of Modern Ion Beam Materials Analysis, 2nd edn. (Materials Research Society, Pittsburgh, 2009). ISBN 978-1-60511-215-2
D. Endisch, H. Sturm, F. Rauch, Nucl. Instrum. Methods B84, 380 (1994)
M. Wilde, K. Fukutani, Surf. Sci. Rep. 69, 196 (2014)
J.F. Ziegler, SRIM, The Stop** and Range of Ions in Matter (2013), http://www.srim.org/SRIM/Compounds.htm
J.F. Ziegler, M.D. Ziegler, J.P. Biersack, Nucl. Instrum Methods B268, 818 (2010) http://www.srim.org
K.M Horn, W.A. Lanford, Nucl. Instrum Methods B34, 1 (1988)
G. Imbriani, R.J. deBoer, A. Best, M. Couder, G. Gervino, J. Görres, P.J. LeBlanc, H. Leiste, A. Lemut, E. Stech, F. Strieder, E. Uberseder, M. Wiescher, Phys. Rev. C 85, 065810 (2012)
B. Maurel, G. Amsel, Nucl. Instrum Methods 218, 159 (1983)
W. Rudolph, C. Bauer, K. Brankhoff, D. Grambole, R. Grötzschel, C. Heiser, F. Herrmann, Nucl. Instrum Methods B15, 508 (1986)
T. Osipowiez, K.P. Lieb, S. Brüssermann, Nucl. Instrum Methods BI8, 232 (1987)
G. Amsel, B. Maurel, Nucl. Instrum Methods 218, 183 (1983)
L. Borucki, H.W. Becker, F. Gorris, S. Kubsky, W.H. Schulte, C. Rolfs, Eur. Phys. J. A 5, 327 (1999)
W.H. Schulte, H. Ebbing, S. Wüstenbecker, H.W. Becker, M. Berheide, M. Buschmann, C. Rolfs, G.E Mitchell, J.S. Schweitzer, Nucl. Instrum Methods B71, 291 (1992)
W.E. Lamb, Phys. Rev. 55, 190 (1939)
J.M. Donhowe, J.A. Ferry, W.G. Monrad, R.G. Herb, Nucl. Phys. A102, 383 (1967)
M. Zinke-Allmang, O. Kruse, Nucl. Instrum Methods B90, 579 (1994)
K.M Horn, W.A. Lanford, Nucl. Instrum Methods B29, 609 (1988)
F. Traeger, M. Kauer, Ch. Wöll, D. Rogalla, H.W. Becker, Phys. Rev. B 84, 075462 (2011)
N. Bohr, K. Dan Viden, Selsk. Math. Fys. Medd. 18, 1 (1948)
A. Ludwig, J. Cao, B. Dam, R. Gremaud, Appl. Surf. Sci. 254, 682 (2007)
A. Ludwig, J. Cao, A. Savan, M. Ehmann, J. Alloys Compd. 446–447, 516 (2007)
G. Hirth, D.L. Kohlstedt, Earth Planet. Sci. Lett. 144, 93 (1996)
M. Murakami, K. Hirose, H. Yurimoto, S. Nakashima, N. Takafuji, Science 295, 1885 (2002)
D.R. Bell, G.R. Rossmann, J. Maldner, D. Endisch, F. Rauch, J. Geophys. Res. 108(B2), 2105 (2003)
J. Gose, P. Reichart, G. Dollinger, E. Schmädicke, Am. Mineral. 93, 1613 (2008)
J.-P. Thomas, M. Fallavier, J. Tousset, Nucl. Instrum. Methods 187, 573 (1981)
C. Le Guillou, H.G. Changela, R. Dohmen, T. Müller, A.J. Brearley, C. Vollmer, D. Rogalla, H.W. Becker, Contribution to the 45th Lunar and Planetary Science Conference, The Woodlands
C. Le Guillou, R. Dohmen, D. Rogalla, T. Müller, C. Vollmer, H.-W. Becker, Chem. Geol. Chem. Geol. 412 (2015) 179
J. Maldner, F. Rauch, AIP Conf. Proc. 392, 689 (1997)
Acknowledgements
We would like to thank F. Traeger, S. Chakraborty and C. Le Guillou for fruitful discussions and comments on the manuscript. We are also thankful to M. Kieschnick and A. Ludwig for providing data not yet published.
Author information
Authors and Affiliations
Corresponding author
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 2016 Springer International Publishing Switzerland
About this chapter
Cite this chapter
Becker, HW., Rogalla, D. (2016). Nuclear Reaction Analysis. In: Fritzsche, H., Huot, J., Fruchart, D. (eds) Neutron Scattering and Other Nuclear Techniques for Hydrogen in Materials. Neutron Scattering Applications and Techniques. Springer, Cham. https://doi.org/10.1007/978-3-319-22792-4_11
Download citation
DOI: https://doi.org/10.1007/978-3-319-22792-4_11
Published:
Publisher Name: Springer, Cham
Print ISBN: 978-3-319-22791-7
Online ISBN: 978-3-319-22792-4
eBook Packages: Chemistry and Materials ScienceChemistry and Material Science (R0)