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Article
Laser-induced spectral broadening and hole-burning in rare earth doped crystals and coherent optical spectroscopy for frequency upconversion
The excitation spectra for linear fluorescence and for frequency upconversion are recorded in Er3+ doped crystal Er:YAG. An excitation induced spectral broadening and hole-burning are shown to appear at the reson...
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Article
Quantum chemical construction of a reduced reaction Hamiltonian and T 1 -relaxation and pure T 2 -dephasing rates for the proton transfer in 3-chlorotropolone
Separating multidimensional problems into that of a relevant system which is coupled to a bath of harmonic oscillators is a common concept in condensed phase theory. Focusing on the specific problem of intramo...
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Chapter and Conference Paper
Femtosecond Optical Spectroscopies of Solvated Polyatomic Molecules
A multimode Brownian oscillator model is developed for third order nonlinear optical spectroscopies in condensed phases, taking into account molecular dynamics of coherent nuclear motions of the absorber and t...