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Article
Efficient amplification of sub-picosecond pulses of a non-CW dye laser
Efficient amplification in a dye laser amplifier is investigated theoretically and experimentally. A five-level rate equation approach is considered including rotational relaxation of the dye molecules. The ef...
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Article
Collective modes — An analytical model for active mode locking in the transient case
A novel concept is presented for the pulse generation in the linear regime of an actively loss modulated laser. Introducing collective laser modes, the frequency detuning of the modulator and the statistical i...
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Article
Polarization effects of picosecond CARS in liquids
Coherent Raman scattering of delayed probing pulses after ultrafast excitation is investigated under generalized polarization conditions. Three factors are shown to contribute to the scattering signal:
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Article
Effect of non-exponential dephasing on near-resonant stimulated Raman scattering
The gain characteristics and spectral properties of transient stimulated Raman scattering are investigated in the non-resonant case. For moderate amplification of the input Stokes pulses by a factor of approxi...
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Article
Off-resonant excitation of molecular vibrations in liquids, investigated by picosecond probe scattering
The coherent excitation of molecular vibrations in liquids via off-resonant stimulated Raman amplification is shown to consist of two parts with vastily different spectral and temporal properties. One componen...
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Article
New results on vibrational population decay in simple liquids
The population lifetimes of the symmetric CH2-stretching mode of several methylene halides were measured after infrared excitation by spontaneous anti-Stokes Raman scattering of delayed picosecond probe pulses. D...
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Article
Picosecond pulses and applications
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Article
Vibrational relaxation of dye molecules investigated by ultrafast induced dichroism
Theoretical and experimental data are presented on the propagation of picosecond pulses in weakly excited dye solutions. It is shown that the so called “coherence peak” of the induced dichroism observed at sho...
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Article
New results on ultrafast coherent excitation of molecular vibrations in liquids
Coherent Raman probe scattering experiments are performed to study dynamical processes of polyatomic liquids at 300 K. For single homogeneous transitions the dephasing timeT 2 is readily obtained from time resolv...