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Preparation and enhanced off-resonance optical nonlinearities of CdS-capped gold nanoparticles embedded in BaTiO3 thin films

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Abstract

A simple approach has been developed for the synthesis of Au@CdS core-shell nanoparticles by a direct self-assembling process. Stable Au@CdS composite colloids were prepared by thiourea, as a double-functional reagent that acted as the linkage agent between Cd2+ ions and gold nanoparticles. The CdS-capped gold composite nanoparticles were successfully integrated into BaTiO3 films. A significant enhancement of third-order nonlinear optical susceptibility in the Au@CdS nanoparticles with core-shell structure is reported. To compare the effect of enhanced nonlinear response, single gold or CdS nanoparticles embedded in BaTiO3 films were also prepared.

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Authors and Affiliations

  1. State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, People’s Republic of China

    Yong Yang, Jianlin Shi, Hangrong Chen, Weiming Huang & Ye Liu

  2. Physics Department, National Key Laboratory of Applied Surface Physics, Fudan University, Shanghai, People’s Republic of China

    Shugang Dai

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  1. Yong Yang
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  2. Jianlin Shi
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  3. Hangrong Chen
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  4. Shugang Dai
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  5. Weiming Huang
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  6. Ye Liu
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Correspondence to Jianlin Shi.

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Yang, Y., Shi, J., Chen, H. et al. Preparation and enhanced off-resonance optical nonlinearities of CdS-capped gold nanoparticles embedded in BaTiO3 thin films. Journal of Materials Research 17, 2802–2808 (2002). https://doi.org/10.1557/JMR.2002.0407

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  • DOI: https://doi.org/10.1557/JMR.2002.0407

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