Log in

Origin and geological control of desorbed gas in multi-thin coal seam in the Wujiu depression, Hailar Basin, China

  • Research Article
  • Published:
Frontiers of Earth Science Aims and scope Submit manuscript

Abstract

To understand the natural gas characteristics of multi-thin coal seam, this study selected the desorbed gas of coal seams in different layers of Well A in the Wujiu depression, Hailar Basin in northeast Inner Mongolia. The results show that the heavy hydrocarbon content of desorbed gas increases significantly with the increasing depth. Methane carbon (δ13C1) and ethane carbon (δ13C2) isotope values are vertically become heavier downwards, while the \({\delta ^{13}}{{\rm{C}}_{{\rm{C}}{{\rm{O}}_{\rm{2}}}}}\) values did not change significantly. The kerogen is close to the III−II mixed type with the source rocks mainly deposited in a shore/shallow lake or braided-river delta front, and the gas produced has certain characteristics of oil associated gas. However, the characteristics of oil associated gas produced by the organic formed in the shallow-water environment (braided-river delta plain) are not obvious. The sandstone pore and fracture systems interbedded with multi-thin coal seam are well developed. And it is conducive to the migration of methanogenic micro-organisms to coal seams via groundwater, making it easier to produce biogenic gas under this geological condition. During the burial evolution of coal-bearing strata in the study area, when the burial depth reaches the maximum, there are significant differences in the paleotemperature experienced by different vertical coal seams, caused by a high-paleogeothermal gradient, increasing the δ13C2 of desorbed gas with increasing depth. The above research indicates that there is less biogenic gas in the multi-thin coal seams with relatively developed mudstone, and the multi-thin coal seams with relatively developed sandstones have obvious biogenic gas characteristics. Therefore, for the exploration and development of biogenic gas in low-rank multi-thin coal seams, it is necessary to give priority to the layer with high sandstone content.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Subscribe and save

Springer+ Basic
EUR 32.99 /Month
  • Get 10 units per month
  • Download Article/Chapter or Ebook
  • 1 Unit = 1 Article or 1 Chapter
  • Cancel anytime
Subscribe now

Buy Now

Price includes VAT (Germany)

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Bannerjee M, Mendhe V A, Kamble A D, Varma A K, Singh B D, Kumar S (2021). Facets of coalbed methane reservoir in East Bokaro Basin, India. J Petrol Sci Eng, 208: 109255

    Google Scholar 

  • Bao Y, Wei C, Neupane B (2016). Generation and accumulation characteristics of mixed coalbed methane controlled by tectonic evolution in Liulin CBM field, eastern Ordos Basin, China. J Nat Gas Sci Eng, 28: 262–270

    Google Scholar 

  • Bernard B B, Brooks J M, Sackett W M (1978). Light hydrocarbons in recent Texas continental shelf and slope sediments. J Geophys Res, 83(C8): 4053–4061

    Google Scholar 

  • Boreham C J, Golding S D, Glikson M (1998). Factors controlling the origin of gas in Australian Bowen Basin coals. Org Geochem, 29(1–3): 347–362

    Google Scholar 

  • Chen Y, Zhang B, Qin Y, Li Z, Yang Z, Wu C, Cao C (2020). Differences in CH4 and C2H6 carbon isotopic compositions from open and closed pores in coal: implications for understanding the two-stage δ13C shift during canister desorption. Int J Coal Geol, 230: 103586

    Google Scholar 

  • Clayton C J, Hay S J, Baylis S A, Dipper B (1997). Alteration of natural gas during leakage from a North Sea salt diapir field. Mar Geol, 137(1–2): 69–80

    Google Scholar 

  • Dai J, Gong D, Ni Y, Huang S, Wu W (2014). Stable carbon isotopes of coal-derived gases sourced from the Mesozoic coal measures in China. Org Geochem, 74: 123–142

    Google Scholar 

  • Feng Z, Ren Y, Zhang X, Zhang J, Dong W, Li C, Li F (2004). Law of oil gas distribution in Hailar Basin and orientation for exploration at next stage. China Petrol Explor, 4: 19–22+1 (in Chinese)

    Google Scholar 

  • Gao L, Mastalerz M, Schimmelmann A (2020). The origin of coalbed methane. In: Thakur P, Schatzel S J, Aminian K, Rodvelt G, Mosser, M M, D’Amico, J S, eds. Coal Bed Methane (2nd ed), Elsevier: 3–34

  • Gonçalves P A, Morgado A, Filho J G M, Mendonça J O, Flores D (2021). Paleoenvironmental variations in a sedimentary Jurassic sequence from Lusitanian Basin (Portugal). Intern J Coal Geo, 247: 103858

    Google Scholar 

  • Harris S H, Smith R L, Barker C E (2008). Microbial and chemical factors influencing methane production in laboratory incubations of low-rank subsurface coals. Intern J Coal Geo, 76(s1–2): 46–51

    Google Scholar 

  • Hu Y, Yuan Y, Yan Z, Liao Y, Liu X, He R, Zhang H, Guan J (2009). Isolation and phylogenetic analysis of a methanogen with wide growth pH range. Chin J Appl Environ Biol, 15(04): 554–558 (in Chinese)

    Google Scholar 

  • Johnson R L, Scott M P, Jeffrey R G (2010). Evaluating hydraulic fracture effectiveness in a coal seam gas reservoir from surface tiltmeter and microseismic monitoring. J Pet Technol, 63(03): 59–62

    Google Scholar 

  • Kinnon E C P, Golding S D, Boreham C J, Baublys K A, Esterle J S (2010). Stable isotope and water quality analysis of coal bed methane production waters and gases from the Bowen Basin, Australia. Int J Coal Geol, 82(3–4): 219–231

    Google Scholar 

  • Kotarba M J (2001). Composition and origin of coalbed gases in the Upper Silesian and Lublin basins, Poland. Org Geochem, 32(1): 163–180

    Google Scholar 

  • Li J, Shao L, Sun B (2019). Sequence-palaeogeography and coal accumulation of the Damoguaihe Formation in the Wujiu mining area, Yakeshi Coalfield, Hailar Basin. J China Coal Soc, 44(S2): 610–619 (in Chinese)

    Google Scholar 

  • Li G, Qin Y, Yao Z, Hu W (2021a). Differentiation of carbon isotope composition and stratabound mechanism of gas desorption in shallow-buried low-rank multiple coal seams: case study of Well DE-A, Northeast Inner Mongolia. Nat Resour Res, 30(2): 1511–1526

    Google Scholar 

  • Li G, Qin Y, Zhou X, Zhang Y, Hu W (2021b). Comparative analysis of the pore structure of fusain in lignite and high-volatile bituminous coal. J Nat Gas Sci Eng, 90: 103955

    Google Scholar 

  • Li G, Qin Y, Zhang M, Wang B, Li J (2022). Microporous structure and gas adsorption model of fusain in lignite. Fuel, 309: 122186

    Google Scholar 

  • Li S, Hegner E, Yang Y, Wu J, Chen F (2014). Age constraints on late Mesozoic lithospheric extension and origin of bimodal volcanic rocks from the Hailar basin, NE China. Lithos, 190–191: 204–219

    Google Scholar 

  • Li Y, Tang D, Fang Y, Xu H, Meng Y (2014). Distribution of stable carbon isotope in coalbed methane from the east margin of Ordos Basin. Sci China Earth Sci, 57(8): 1741–1748

    Google Scholar 

  • Li Y, Zhang C, Tang D, Gan Q, Niu X, Wang K, Shen R (2017). Coal pore size distributions controlled by the coalification process: an experimental study of coals from the Junggar, Ordos and Qinshui Basins in China. Fuel, 206: 352–363

    Google Scholar 

  • Liu J, Shi G, Guo Q (1994). Quantitative method of recovering thermal evolution history with apatite fission track. Petrol Explor Dev, 04: 15–18+116 (in Chinese)

    Google Scholar 

  • Lu S, Feng G, Shao M, Li J, Xue H, Wang M, Chen F, Li W, Pang X (2021). Kinetics and fractionation of hydrogen isotopes during gas formation from representative functional groups. Petrol Sci, 18(4): 1021–1032

    Google Scholar 

  • Monthioux M, Landais P, Monin J C (1985). Comparison between natural and artificial maturation series of humic coals from the Mahakam delta. Indonesia, 8(4): 0–292

    Google Scholar 

  • Mukhopadhyay P K, Wade J A, Kruge M A (1995). Organic facies and maturation of Jurassic/Cretaceous rocks, and possible oil-source rock correlation based on pyrolysis of asphaltenes, Scotian Basin, Canada. Org Geochem, 22(1): 85–104

    Google Scholar 

  • Papendick S L, Downs K R, Vo K D, Hamilton S K, Dawson G K W, Golding S D, Gilcrease P C (2011). Biogenic methane potential for Surat Basin, Queensland coal seams. Int J Coal Geol, 88(2–3): 123–134

    Google Scholar 

  • Qin Y, Shen J, Shen Y, Li G, Fan B, Yao H (2019). Geological causes and inspirations for high production of coal measure gas in Surat Basin. Acta Petrol Sin, 40(10): 1147–1157 (in Chinese)

    Google Scholar 

  • Queensland Government (2021) Production and reserve statistics. Available at Queensland Government website

  • Schoell M (1980). The hydrogen and carbon isotopic composition of methane from natural gases of various origins. Geochim Cosmochim Acta, 44(5): 649–661

    Google Scholar 

  • Schoell M (1983). Genetic characterization of natural gases. AAPG Bull, 67: 2225–2238

    Google Scholar 

  • Scott A R, Kaiser W R (1994). Thermogenic and Secondary biogenic gases, San Juan Basin, Colorado and New Mexico-Implications for Coalbed Gas Producibility. AAPG Bull, 78(8): 1186–1209

    Google Scholar 

  • Shang N (2020). Coalification and structural control of Damoguaihe Formation in Wujiu Depression, Inner Mongolia, China. Dissertation for the Doctoral Degree. Xuzhou: China University of Mining and Technology (in Chinese)

    Google Scholar 

  • Shields D, Bianchi V, Esterle J (2017). A seismic investigation into the geometry and controls upon alluvial architecture in the Walloon Subgroup, Surat Basin, Queensland. Aust J Earth Sci, 64(4): 455–469

    Google Scholar 

  • Souza I M S, Cerqueira J R, Garcia K S, Ribeiro H J P S, Oliveira O M C, Queiroz A F S, Teixeira L S G (2021). Geochemical characterization and origin of kerogens from source-rock of Devonian in the Amazonas Basin, Brazil. J S Am Earth Sci, 111: 103437

    Google Scholar 

  • Su N, Zhu G, Wu X, Yin H, Lu Y, Zhang S (2021). Back-arc tectonic tempos: records from Jurassic-Cretaceous basins in the eastern North China Craton. Gondwana Res, 90: 241–257

    Google Scholar 

  • Su X, Xu Y, Wu Y, **a D, Chen X (2011). Effect of salinity and pH on biogenic methane production of low-rank coal. J China Coal Soc, 36(08): 1302–1306 (in Chinese)

    Google Scholar 

  • Tamamura S, Murakami T, Aramaki N, Ueno A, Tamazawa S, Badrul A, Haq S, Igarashi T, Aoyama H, Yamaguchi S, Kaneko K (2019). The role of meteoric water recharge in stimulating biogenic methane generation: a case study from the Tempoku Coal Field, Japan. Int J Coal Geol, 202: 14–26

    Google Scholar 

  • Tang Y, Gu F, Wu X, Ye H, Yu Y, Zhong M (2018). Coalbed methane accumulation conditions and enrichment models of Walloon Coal measure in the Surat Basin, Australia. Nat Gas Indust B, 5(3): 235–244

    Google Scholar 

  • Wang A, Shao P, Lan F, ** H (2018). Organic chemicals in coal available to microbes to produce biogenic coalbed methane: a review of current knowledge. J Nat Gas Sci Eng, 60: 40–48

    Google Scholar 

  • Wang B, Li J, Zhang Y, Wang H, Liu H, Li G, Ma J (2009). Geological characteristics of low rank coalbed methane, China. Pet Explor Dev, 36(1): 30–34

    Google Scholar 

  • Wang B, Qin Y, Shen J, Wang G, Zhang Q, Liu M (2019). Experimental study on water sensitivity and salt sensitivity of lignite reservoir under different Ph. J Petrol Sci Eng, 172: 1202–1214

    Google Scholar 

  • Wang F, Zhou X, Zhang L, Ying J, Zhang Y, Wu F, Zhu R (2006). Late Mesozoic volcanism in the Great **ng’an Range (NE China): timing and implications for the dynamic setting of NE Asia. Earth Planet Sci Lett, 251(1–2): 179–198

    Google Scholar 

  • Wang X, Zhao Y (2020). The time-temperature-maturity relationship: A chemical kinetic model of kerogen evolution based on a developed molecule-maturity index. Fuel, 278: 118264

    Google Scholar 

  • Wang Y, Zhang F, Zou Y, Sun J, Lin X, Liang T (2018). Oil source and charge in the Wuerxun Depression, Hailar Basin, northeast China: a chemometric study. Mar Pet Geol, 89(3): 665–686

    Google Scholar 

  • Wei Q, Hu B, Li X, Feng S, Xu H, Zheng K, Liu H (2021). Implications of geological conditions on gas content and geochemistry of deep coalbed methane reservoirs from the Panji Deep Area in the Huainan Coalfield, China. J Nat Gas Sci Eng, 85: 103712

    Google Scholar 

  • Whiticar M J, Faber E, Schoell M (1986). Biogenic methane formation in marine and freshwater environments: CO2 reduction vs. acetate fermentation—isotope evidence. Geochim Cosmochim Acta, 50(5): 693–709

    Google Scholar 

  • Whiticar M J (1999). Carbon and hydrogen isotope systematics of bacterial formation and oxidation of methane. Chem Geol, 161(1–3): 291–314

    Google Scholar 

  • Yuan M, Lyu S, Wang W, Xu F, Yan X (2022). Macrolithotype controls on natural fracture characteristics of ultra-thick lignite in Erlian Basin, China: implication for favorable coalbed methane reservoirs. J Petrol Sci Eng, 208: 109598

    Google Scholar 

  • Zhang B, Chen Y (2020). Particle size effect on pore structure characteristics of lignite determined via low-temperature nitrogen adsorption. J Nat Gas Sci Eng, 84: 103633

    Google Scholar 

  • Zhang J (2020). Hydrogeological conditions of controlling gas in coal measures in Wujiu Depression. Dissertation for the Doctoral Degree. Xuzhou: China University of Mining and Technology (in Chinese)

    Google Scholar 

  • Zhang S, Zhang X, Li G, Liu X, Zhang P (2019). Distribution characteristics and geochemistry mechanisms of carbon isotope of coalbed methane in central-southern Qinshui basin, China. Fuel, 244: 1–12

    Google Scholar 

  • Zhang Y, Li S, Tang D, Zhao X, Zhu S, Ye J (2020). Structure- and hydrology-controlled isotopic coupling and heterogeneity of coalbed gases and co-produced water in the Yanchuannan block, southeastern Ordos Basin. Int J Coal Geol, 232: 103626

    Google Scholar 

Download references

Acknowledgements

We would like to thank the National Natural Science Foundation of China (Grant Nos. 42130802, 42002193, and 42002186) and researchers Yanqiu Zhang, Wutao Hu, Haitao Lin, and Fengchun Li from Inner Mongolia Coal Geology Bureau for their help in sample acquisition. Thank anonymous reviewers for their valuable suggestions. Furthermore, we would like to thank Master Zhen Zhang from China University of Mining and Technology for his help in field work.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Yong Qin.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Li, G., Qin, Y., Song, X. et al. Origin and geological control of desorbed gas in multi-thin coal seam in the Wujiu depression, Hailar Basin, China. Front. Earth Sci. 17, 58–70 (2023). https://doi.org/10.1007/s11707-022-0994-1

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11707-022-0994-1

Keywords

Navigation