Abstract
This paper presents the Heavy Metals Eulerian Transport (HMET) model and simulation results for Europe for 1985. The HMET model takes into account emission, atmospheric transport and deposition of As, Cd, Pb and Zn computed on the EMEP grid system. Meteorological inputs consist of the velocity field at 925 hPa, precipitation and mixing height. Velocity field and precipitation are updated every 6 hr during the model run. New values of mixing height are available every 24 hr. The dry deposition velocities for each metal are variable in space and depend on the particle distribution function for each particular metal. Wet deposition is proportional to the precipitation intensity for the previous 6 hr and a constant scavenging ratio. Model equations are solved by means of the positive definite pseudospectral method which provides accurate numerical solutions for the advection problem. Comparison of the model results with available observations for 1985 indicate a good agreement for Cd and Pb, sufficient egreement for As and serious underestimation for Zn. Since the number of available observations for heavy metals in Europe in 1985 is relatively small, the model results presented in this paper should be considered as preliminary. However, the HMET model performance in computing these results shows that it can be easily and efficiently used as an operational tool and is especially useful for estimating transboundary transport of heavy metals in Europe.
Similar content being viewed by others
References
Alcamo, J., Bartnicki, J., Olendrzyński, K.: 1991, in H. van Dop and G. Steyn, (eds.), Air Pollution Modeling and Its Application VIII, Plenum Press, New York, pp. 391–400.
Alcamo, J., Bartnicki, J., Olendrzyński, K., and Pacyna, J.: 1992, Atmospheric Environment 26a, 3355.
Amundsen, J. E., Hansen, J. E., Semb, A., and Stainnes, E.: 1992, Atmospheric Environment 26a, 1309.
Barrie, L. A.: 1988, J. Geophys, Res. 93, D4, 3773.
Barrie, L. A. and Schemenauer, R. S.: 1989, in J. M. Pacyna, and B. Ottar, (eds.), Control and Fate of Atmospheric Trace Metals, Kluwer Acad. Publ., Dordrecht, pp. 203–232.
Bartnicki, J.: 1990, Environmental Software 34, 187.
Bartnicki, J.: 1991a, in H. van Dop and G. Steyn, (eds.), Air Pollution Modeling and Its Application VIII, Plenum Press, New York, pp. 339–348.
Bartnicki, J.: 1991b, ‘An Application of the PDPS Method to Transboundary Air Pollution Modeling’, Proceedings, 2nd IUPPA Regional Conference on Air Pollution, Seoul, Korea, Sept. 1991. Vol. 2, pp. 203–210.
Carras, J. N. and Williams, J. N.: 1981, Atmospheric Environment 15, 2205.
Chan, W. H., Tang, A. J. S. Chung, D. H. S., and Lusis, M. A.: 1986, Water, Air, and Soil Pollut. 29, 373.
Christensen, O. and Prahm, L. P: 1976. Journal of Applied Meteorology 15, 1284.
Chock, D. P.: 1991, Atmospheric Environment 24A(8), 853.
Cooley, J. W. and Tukey, J. W.: 1965, Math. Comp. 19, 297.
Dulac, F., Baut-Menard, P., Ezet, U., Melki, S. and Bergametti, G.: 1989, Tellus 41B(8), 362.
Eliassen, A. and Saltbones, J.: 1983, Atmospheric Environment 17(8), 1457.
Gazdag, J.: 1973, Journal of Computational Physics, 13, 100.
Galloway, J., Thornton, J., Norton, S., Volchok, H. and McLean, R.: 1982, Atmospheric Environment 16(7), 1677.
Georgii, H. W., Perseke, C. and Rohbock, E.: 1983, in Beilke, S. and Elshout, A., (eds.), Acid Deposition, D. Reidel Publ. Co. Dordrecht, pp. 142–148.
Gravenhorst, G., Höfken, K. and Georgii, H. W.: 1983, in Beilke, S. and Elshout, A., (eds.), Acid Deposition, D. Reidel Publ. Co. Dordrecht, pp. 155–171.
Gydesen, H., Pilegaard, K., Rasmussen, L. and Rühling, Å: 1983, ‘Moss Analyses Used as a Means of Surveying the Atmospheric Heavy-metal Deposition in Sweden, Denmark and Greenland in 1980’, Bulletin PM 1670, 44 pp.
Heffter, J. L.: 1965, Journal of Applied Meteorology 4, 153.
Högström, U.: 1979, Atmospheric Environment 13, 295.
Iversen, T., Halvorsen, N. E., Mylona, S. and Sandnes, H.: 1991, Calculated Budgets for Airborne Acidifying Components in Europe, 1985, 1987, 1988, 1889 and 1990. EMEP MSC-W Report 1/91.
Jaarsveld van, J. A., van Aalst, R. M. and Onderdelinden, D.: 1986, Deposition of Metals from the Atmosphere to the North Sea: Model Calculations. National Institute for Public Health and Environmental Protection (RIVM), Bilthoven, The Netherlands, Report 842015002.
Jaarsveld van J. A.: 1991, Estimating Atmospheric Input of Trace Metals to the North Sea; Methods and results, Proceedings of the 19th NATO/CCMS International Technical Meeting on Air Pollution Modeling and Its Application — Crete, Greece.
Krell, U. and Roeckner, E.: 1988, Atmospheric Environment 17, 375.
Kristensen, L., Jensen, N. O. and Petersen, E. L.: 1981: Atmospheric Environment 15, 837.
Lahman, E., Munari, S., Amicarelli, V. and Abbatichio, P.: 1986, Heavy Metals: Identification of Air Quality and Environmental problems in the European Community. Vol. 1. EUR 10678. CEC Brussels.
Mészáros, A., Friedland, A. J., Haszpra, L., Mészáros, E., Lászity, A. and Horváth, Z.: 1987, in Lindberg, S. and Hutchinson, T., (eds.), Heavy Metals in the Environment, CEP Consultants, Edinburgh.
Norwegian SPCA (State Pollution Control Authority): 1986, ‘Norwegian Monitoring Programme for Long Range Transported air Pollutants. TA-606. Report 230/86.
Nriagu, J. O.: 1988, Environmental Pollution 50, 139.
Nriagu, J. O. and Pacyna, J. M.: 1988, Nature 333, 134.
Nriagu, J. O.: 1991, in Pacyna, J. M. and Ottar, B. (eds.), Control and Fate of Atmospheric Trace Metals, Kluwer Acad. Publ., Dordrecht, pp. 3–14.
Ottar, B., Lindberg, S. E., Voldner, E., Lindqvist, O., Mayer, R., Semb, A., Steinnes, E. and Watt J.: 1989, in Pacyna, J. M. and Ottar, B. (eds.), Control and Fate of Atmospheric Trace Metals, Kluwer Acad. Publ. Dordrecht, pp. 365–372.
Pacyna, J. M.: 1988, ‘Atmospheric Lead Emissions in Europe in 1985’. NILU Report OR 18/88. Norwegian Institute for Air Research. Lillestrøm.
Pacyna, J. M.: 1991, personal communication.
Pacyna, J. M. and Münch, J.: 1988, ‘Atmospheric Emissions of Arsenic, Cadmium, Mercury and Zinc in Europe in 1982’. NILU Report OR 17/88. Norwegian Institute for Air Research. Lillestrøm.
Pacyna, J. M. and Ottar, B.: 1985, Atmospheric Environment 19, 2109.
Pacyna, J. M. Ottar, B., Tamza, U. and Meanhaut, W.: 1985, Atmospheric Environment 19, 857.
Pacyna, J. M., Bartonova, A., Cornille, P. and Meanhaut, W.: 1989, Atmospheric Environment 13(1), 107.
PARCOM (Paris Commission): 1986, ‘Results of Coastal Stations in the First Phase of the Pilot Project’. Report ATMOS 4/4/10E.
Pasquill, T.: 1963, em Atmospheric Diffusion, Van Nostrand-Rheinhold, London.
Petersen, G., Weber, H. and Grass, H.: 1989, in Pacyna, J. M. and Ottar, B. (eds.), Control and Fate of Atmospheric Trace Metals, Kluwer Acad. Publ., Dordrecht, pp. 57–84.
Rühling Å., Pilegaard, K., Mäkinen. A. and Steinnes, E. (1987): ‘Survey of Atmospheric Heavy Metal Deposition in the Nordic Countries in 1985 — Monitored by Moss Analysis’. NORD 187:21, pp. 44.
Rühling, Å., Pilegaard, K., Brumelis, G., Goltsova, N., Kvietkus, K., Kubin, E., Liiv, S., Magnússon, S., Mäkinen, A., Pilegaard, K., Rasmussen, L., Sandar, E. and Steinnes, E. (1992): ‘Atmospheric Heavy Metal Deposition in Northern Europe 1990’ NORD 1992:12, pp. 41.
Sehmel, G. A.: 1980, Atmospheric Environment 14, 983.
Smith, F. B., and Hunt, R. D.: 1978, Atmospheric Environment 12, 461.
Steinnes, E.: 1989, in Pacyna, J. M. and Ottar, B. (eds.), Control and Fate of Atmospheric Trace Metals, Kluwer Acad. Publ., Dordrecht, pp. 321–388.
Ross, H.: 1987, Water, Air, and Soil Pollut. 36, 349.
WHO (World Organization, Regional Office for Europe): 1989, Air Quality Guidelines for Europe, Copenhagen.
Wiersma, G. B. and Davidson, C. I.: 1986, in Nriagu, J. O. and Davidson, C. I. (eds.), Toxic Metals in the Atmosphere, John Wiley, New York, pp. 201–266.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Bartnicki, J. An Eulerian model for atmospheric transport of heavy metals over Europe: Model description and preliminary results. Water Air Soil Pollut 75, 227–263 (1994). https://doi.org/10.1007/BF00482939
Received:
Accepted:
Issue Date:
DOI: https://doi.org/10.1007/BF00482939